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MAGAZINE
f e at u r e s
8 Renewable Hydrogen—
Economically Viable
37 The Future Is Present
in California
Integration into the U.S. Delivering on the promise
transportation sector. of fuel cell-powered
Jennifer Kurtz, Mike Peters, transportation.
Matteo Muratori, and Chris Gearhart Andrew Martinez
26 Government Policies
Help Promote Clean
55 The Island
Hydrogen Project
Transportation in India Electrolytic generated Mission Statement: IEEE Electrification Maga-
Proton-exchange membrane hydrogen for automotive zine is dedicated to disseminating information on
fuel cells for vehicles. and maritime applications. all matters related to microgrids onboard electric
vehicles, ships, trains, planes, and off-grid applica-
Bandi Mallikarjuna Reddy, Silviu Nistor, Stephen Carr, tions. Microgrids refer to an electric network in a
Paulson Samuel, and and Mahesh Sooriyabandara car, a ship, a plane or an electric train, which has a
Narapureddy Siva Mohan Reddy limited number of sources and multiple loads. Off-
grid applications include small scale electricity sup-
ply in areas away from high voltage power net-
works. Feature articles focus on advanced con-
cepts, technologies, and practices associated with
all aspects of electrification in the transportation
and off-grid sectors from a technical perspective in
synergy with nontechnical areas such as business,
d e pa r t m e n t s & c o l u m n s environmental, and social concerns.
Powering
Editor, Electric Trains Faraday Future
Ganz-Skoda California, USA
Hungary silva.hiti@ff.com
tamas.ruzsanyi@ieee.org
Transportation with
Eduard Muljadi
Eduardo Pilo de la Fuente Editor, Electric Vehicles
Editor, Electric Trains Auburn University
EPRail Research Alabama, USA
Syed A. Hossain
Editor, Electric Planes
Jose Conrado Martinez GE Aviation
Editor, Electric Trains Ohio, USA
Directcion de Estrategia syed.hossain@ge.com
By Eduard Muljadi and Syed Hossain y Desarrollo
Spain Kaushik Rajashekara
jcmartinez@adif.es Editor, Electric Planes
University of Houston
Suryanarayana Doolla Texas, USA
ransportation sectors are currently Editor, Microgrid ksraja@central.uh.edu
BENDER INC
1-800-356-4266
www.bender.org
technology leaders
By Chris Gearhart
his is an exciting time the hydrogen economy, which could selves have improved. FC costs have
Electrification of Figure 1. The modeled cost of a PEM FC system based on the projection to high-volume man-
Heavy-Duty Vehicles ufacturing (500,000 units per year). (Data from the National Renewable Energy Laboratory.)
It is not just about light-duty vehicles
anymore. It never really was; buses
have been a big part of early FC
400
deployments, and hundreds of FC
buses have been deployed globally 250
and have been shown to be efficient 300
and durable (NREL 2017). However, Monthly Sales
FC Vehicle Sales
May
2016
August
2016
November
2016
March
2017
June
2017
September
2017
December
2017
meet these challenges has grown. The Another significant trend over the increases in manufacturing volume.
negative health impacts of tailpipe past several decades is the growing Over the last few decades, there has
emissions have been, and continue to commitment of governments around been a dramatic increase in other
be, the primary motivation for the the world to reduce the emission of markets for FC systems. Forklifts and
development and deployment of FCEVs greenhouse gases (GHGs). Nearly material-handling applications have
in the United States. These emissions, every country, apart from the United become a big part of the FC market,
in particular, nitrogen oxides, sulfur States, has signed the Paris Climate with more than 15,000 hydrogen FC
oxides, and particulates, are responsi- Accords. Each country that has signed forklifts already deployed or on order
ble for significant health problems, this agreement determines its own (Office of Energy Efficiency and Re
resulting in a large number of prema- contribution to GHG emissions reduc- newable Energy 2017).
ture deaths every year. California has tions and how it will meet this con- Stationary applications of FC
led the way with ambitious clean air tribution. Of these individually systems have also been growing.
targets that have helped drive the determined contributions, 75% in PEM fuel cells have been shown to
development of FCEVs. clude explicit targets to reduce GHG be robust and reliable sources of
Globally, poor air quality in devel- emissions from the transportation stationary and backup power. The
oping countries such as China and sector. As with clean air standards, ability of FC systems to provide reli-
India is a significant and growing developing countries will need to able backup power to add resilience
problem. Although transportation- achieve these GHG emissions reduc- to the electrical grid during extreme
related emissions are not the only tions while transportation energy weather events is going to make
source of these emissions, they are a consumption nearly doubles. This can these systems increasingly valuable.
significant part of the problem. As only be accomplished and sustained A prior analysis of backup power gen-
the economies of developing nations if transportation energy can come eration in the aftermath of Hurri-
grow, the increased demand for auto- from near-zero-carbon-sources. cane Sandy demonstrated this value
mobiles and freight movement will in dramatic fashion (Kurtz et al.
only make these problems more dif- Emerging Market Applications 2015). The combination of high reli-
ficult to address. Furthermore, the Synergies with other industries that ability and the potential to provide
demand in these countries for zero- use FCs and hydrogen are increasing. low-carbon energy has also made
emission vehicles is going to increase The cost of new technologies is these systems desirable as power
as the need to reduce both emis- reduced through a combination of supplies for data centers. Daimler,
sions and vehicle miles traveled research breakthroughs and reduc- Hewlett Packard, and Power Innova-
becomes more prominent. tions in manufacturing costs due to tions have developed prototype FC
systems to power data center
microgrids (Daimler 2017). Conse-
quently, this market has the poten-
tial to create a dramatic increase in
fuel-cell system sales.
12
Contract Price (US$/kWh)
10 Conclusion
There are still many barriers to the
8 widespread adoption of hydrogen
FCEVs, and we cannot say with
6
certainty how soon we will see this
4 widespread adoption happen. But in
US$0.02/kWh response to those who say that
2 hydrogen will always be the technol-
ogy of the future, I would like to sug-
0
gest that they have not been paying
2008 2010 2012 2014 2015
attention to the successes of the last
Year
decade. A large amount has changed
Solar Wind Capacity (Gigawatt) in the past ten years: the technology
has made significant advances, the
economics of renewable hydrogen
Figure 3. Renewable electricity prices have fallen while capacity has grown. (Figure adapted
from B. Pivovar, H2@Scale: “Energy System-Wide Benefits of Increased Hydrogen Implementa- are quickly changing, the recognition
tion,” presented at the Fuel-Cell Seminar, Long Beach, California, 2017.) of the need for alternative energy
& IAS
ieee-powerafrica.org
Renewable
Hydrogen—
Economically Viable
Integration into the he U.S. transportation sector is expected
T
to meet numerous goals in differing applications.
U.S. transportation These goals address security, safety, fuel source,
8 I EEE E l e c t r i f i c a t i on M a gaz ine / March 2018 U.S. Government work not protected by U.S. Copyright.
used and integrating new systems, such as storing renew- i.e., petroleum refining and fertilizer production. Most of
able energy. Overall, there are many combinations of prob- this hydrogen is produced via steam methane reforming,
lems, objectives, and solutions. which is the lowest-cost production method. Hydrogen is
In this article, we focus on one component of a multi- also being used in the United States for mobile and station-
technology strategy: hydrogen. Hydrogen for transportation ary fuel-cell applications. California now has more than 30
applications can reduce emissions without sacrificing per- retail hydrogen-fueling stations for fuel-cell passenger vehi-
formance, be sourced locally via renewable resources, and cles, and these stations dispensed more than 100,000 kg of
support the U.S. economy through jobs and advanced tech- hydrogen in 2016.
nology development. As a flexible energy carrier, hydrogen Fuel-cell electric vehicles (FCEVs) are available for lease
can also support the electric power and industrial sectors. and purchase in limited regions that have hydrogen infra-
With support from the U.S. Department of Energy (DOE) structure, mainly in California but also in some Northeast
Fuel-Cell Technology Office, the National Renewable Energy locations. Hydrogen fuel-cell buses have been operating in
Laboratory (NREL) is demonstrating ways to improve the revenue transit service for more than a decade. Fuel-cell
cost, performance, and durability of hydrogen production, forklifts are in use by a variety of companies because of
infrastructure, and end-use technologies. their demonstrated value in high-demand warehouse
operations, and fuel-cell trucks are in development
A Sustainable Transportation Solution because of performance benefits, including extended
range, short refueling time, and vehicle driving capability
The Questions (e.g., acceleration and power).
When hydrogen is discussed as a sustainable transporta- Steam methane reforming of natural gas is currently
tion solution, the following questions are commonly asked: the most common and lowest-cost method used to pro-
1) Is hydrogen available and feasible in the near term? duce hydrogen; however, there are many options in vari-
2) Why should hydrogen be part of the solution for ous stages of commercial readiness for hydrogen
reducing transportation emissions even if we still pro- production using renewable resources. The most techni-
duce it from natural gas? cally advanced option is through water electrolysis with
3) How will renewable hydrogen be cost effective and renewable electricity. In fact, many renewable resources in
able to meet the transportation demands? the United States, i.e., wind, solar, and biomass, can be
used to produce hydrogen.
The Answers Currently, it is expensive to produce hydrogen renew-
Today, about ten million metric tons of hydrogen are pro- ably via electrolysis, and research and development (R&D)
duced each year for use primarily in industrial applications, is focused on reducing cost through advancing technology,
2017 By Year
Through Q2 170,139 kg
100
2016 109,202 kg
Hydrogen Dispensed (1,000 kg)
2015 27,431 kg
2014 19,738 kg
80
2013 16,335 kg
2012 17,433 kg
2011 8,055 kg
60
2010 2,260 kg
2009 1,910 kg
0 50 100 150 200
40
H2 Dispensed (1,000 kg)
20
0
2009 Q1
Q2
Q3
Q4
2010 Q1
Q2
Q3
Q4
2011 Q1
Q2
Q3
Q4
2012 Q1
Q2
Q3
Q4
2013 Q1
Q2
Q3
Q4
2014 Q1
Q2
Q3
Q4
2015 Q1
Q2
Q3
Q4
2016 Q1
Q2
Q3
Q4
2017 Q1
Q2
Figure 2. Through June 2017, the hydrogen dispensed by quarter (Q) for stations in the evaluation project. (Image courtesy of NREL.)
Natural
Bioreactor Gas Storage CNG Fueling
Biomass CO2 Storage
Pyrolysis
Hydrogen-
Hydrogen Hydrogen Fueled
Electrolyzer Storage Fueling Vehicles
+ –
CNG-Fueled
Vehicles
Other Renewables:
Solar, Geothermal,
Hydro Electric Line
Hydrogen Piping
CO2 Piping
Natural Gas Piping
Figure 3. The various renewable pathway scenarios for hydrogen production. CNG: compressed natural gas. (Image courtesy of NREL.)
Figure 4. The renewable hydrogen production potential relative to gasoline consumption, by county. (Image courtesy of NREL.)
Figure 5. The hydrogen production potential from dominant renewable resources. Total kg of hydrogen per county, normalized by county area.
(Image courtesy of NREL.)
animal manure, and wastewater treatment centers, have sented a roadmap for improving the economics of renew-
lower overall availability, they are usually located close to able hydrogen.
population centers, and this proximity offers good early- So where are we right now with moving renewably
market opportunities to exploit waste resources and limit produced hydrogen molecules into mobile fuel-cell sys-
transportation cost and infrastructure requirements. tems? Dispensing renewably produced hydrogen to
Overall, it is likely that renewable hydrogen will come FCEVs is currently cost prohibitive, and most hydrogen
from a variety of sources, with large opportunities to sup- stations use delivered gas produced at large, centralized
port the integration of renewable electricity sources and steam methane-reforming plants. However, to fully
exploit otherwise-curtailed renewable electricity. realize the benefits of hydrogen fuel-cell vehicles,
renewable hydrogen stations are necessary and, there-
Status of Renewable Hydrogen fore, are a focus for future hydrogen station research
Production Technologies and development.
NREL is pursuing economically viable technology options
for renewable hydrogen production. The results of path- Renewable Hydrogen-Fueling Stations of Today
ways analyses to date suggest there is more than enough There are a few renewable hydrogen stations currently
renewable resources to domestically produce hydrogen for in operation or planned. The California Energy Com-
the U.S. transportation sector, and H2@Scale analysis pre- mission (CEC) helps fund the capital and operation and
Established
Industrial Process
High-Temp
Coal Gasification Electrolysis
with CCS
Central
Figure 6. The near-, mid-, and long-term hydrogen production pathways. CCS: carbon capture sequestration; STCH: solar thermochemical hydro-
gen production; PEC: photoelectrochemical; P&D: production and delivery. (Image courtesy of the DOE Fuel-Cell Technologies Office.)
Power
Generation Value-Added
Applications
Hydrogen/
Electricity
Natural Gas
Wind Grid
Infrastructure
Hydrogen
Hydrogen Vehicle
Solar PV Storage/
Distribution
ortation
Synthetic
Fuels
Transp
CO2
Upgrading
Natural Oil/
Gas/Coal Biomass
Battery N2
Nuclear,
Thermal,
Geothermal, Ammonia/
and More Fertilizer
Hydrogen Metals
Generation Refining
Other
End Use
CO2 ial
ustr
Ind
Figure 7. An illustrative example of the H2@Scale concept (not comprehensive). PV: photovoltaic. (Images courtesy of B. Pivovar et al., 2017.)
Hydrogen Production
via Water
Electrolysis
The benefits of a
solar cell-powered
process.
he recent emergence
T
of the hydrogen (H 2) fuel-
cell electric vehicle (FCEV)
guarantees the benign
nature of the transpor-
tation industry. Several companies, e.g.,
Toyota and Hyundai, have started to com-
mercialize H 2 FCEV with relatively com-
parable properties to meet the renewable
energy-based future. For instance, the Hyundai
Tucson can drive around 400 mi after 3 min of a
simple H 2 charge. Additionally, to keep abreast of
supporting H 2 FCEVs, Germany has decided to help
construct the fueling stations by supporting funding and
restricting oil-based vehicles production.
of Gas-Reforming H2 Production
The fervent research, industrialization, and funding
of FCEVs are due to the belief that they do not produce any acceptable, because FCEVs utilize the H 2-oxygen (O 2) com-
harmful products after H 2 combustion. This is partially bustion reaction for electricity generation, which results in
water (H 2 O) production. However, mass production of H 2 is
currently based on the gas-reforming process (more than
Digital Object Identifier 10.1109/MELE.2017.2784632
Date of publication: 28 February 2018 96% of total H 2 production), which concomitantly produces
+ + + +
PV EC PV dc-dc
VPV VEC VPV VEC EC
Cell Cell Converter
– – – –
Maximum Maximum
Power EC Power Point Power Power Point EC
PPV,max PPV,max
Boost
Operation
Boost Buck Buck
Operation Operation Operation
PV PV
Figure 1. The two configurations of the PV-EC system. (a) A direct coupling for a PV-EC system. (b) A dc–dc converter connection to construct a
PV-conv-EC system. Power-voltage curves of the PV-EC system when (c) VPV,max > VEC,MPPT and (d) VPV,max < VEC,MPPT.
15 ing that PH2 + Pkin is still smaller than PPV,max. Therefore, the
role of converter can help an EC to fully use the PPV,max [Fig-
10 ure 2(c)]. By the MPPT procedure, extra PH2 gain can be
PH2 Pkin expected, indicating a much higher H 2 gain even with
5 same PV and EC systems, as shown by the yellow line in
Figure 2(b). Unless the efficiency of a converter is small
0 0.5 1 1.5 2 enough to reduce the PH2 to a conventional PV-EC system
Voltage (V) without a converter, the converter utilization is important
(a) part needed to maximize the H 2 generation.
25
EC with Good Catalyst The Advantages of a PV-EC System
EC with Bad Catalyst
20 PV I-V Based on the concept suggested in Figure 2, continuous
research has been made to improve the efficiency, sta-
Current (mA)
Higher PH2
15 bleness, scalability and economic viability of a PV-EC
system. For instance, the concept of connecting solar
Smaller
10 cell with H 2 O electrolysis catalysts was suggested by the
PH2
Turner group at National Renewable Energy Laboratory
5 (NREL). This research, also known as PV-PEC system, pro-
vided insight to the researchers to develop PV-EC sys-
0 0.5 1 1.5 2 tem. NREL’s continuous research increased the efficiency
Voltage (V) of the PV-PEC system and recently broke 16% STH effi-
(b) ciency [Figure 3(a)].
25 Additionally, researchers have developed the novel
P configuration: a topology and material designing process
PV
20 ,m to increase the STH efficiency and sustain its stability dur-
ax
=
I× ing photoelectrolysis. For example, the Nocera group pio-
Current (mA)
V
15 neered the compact PV-EC system, known as an artificial
PH2 leaf. Based on the compact configuration and control of
10 Pkin the number of PV cells, his group utilized four series-con-
EC I-V nected silicon PVs and transition metal-based catalysts to
PV I-V
5 achieve 10% STH efficiency [Figure 3(b)].
Extra PH2
To keep abreast of the fast-growing organic and inor-
0 0.5 1 1.5 2 ganic perovskite solar cell, the Gratzel group applied a PV
Voltage (V) and state-of-the-art transition metal-based catalyst for
(c) H 2 O splitting. This research reaps benefits in terms of cost
efficiency because PV and EC materials are famously inex-
Figure 2. An analysis method for understanding the PV-EC system: pensive. Additionally, this system shows 12.3% STH effi-
(a) the H 2 power density ^PH2h and kinetic loss ^Pkinh at a given cur-
ciency, even with less expensive PV and EC materials,
rent-voltage (I-V) curve of the PV and EC and (b) the contrast of PH2
with a good and bad EC catalyst. (c) PH2 and Pkin after the dc–dc which have comparable efficiency with the PV-EC system
converter assistance on (a) (Chang et al. 2017). (Image courtesy of using novel materials.
the American Chemical Society.)
Recently, several PV-EC systems with more than 20%
STH efficiency have been reported. By controlling the sur-
and VPV = VEC, as stated in the intersection of Figures 1(a) face area of an EC and PV, and by applying concentrator on
and 2(a). We could estimate the amount of power stored a PV, the Fuji group reported a PV-EC system with 24.4%
as H 2 as PH2 and the amount of solar-driven electrical STH efficiency [Figure 3(d)]. In 2016, the Jaramillo group
power loss as Ploss. PH2 can be the generated current from broke 30% STH efficiency by utilizing a state-of-the-art
the PV-EC system multiplied by 1.23 V, since chemical catalyst and an extremely efficient tandem solar cell. Not
energy stored as H 2 is as same as the free-energy change only for the subcompartments, they heated the EC and
of a H 2 O-splitting reaction. optimized the light and series connection of each sub-
At a fixed solar cell condition, the catalyst materials compartment to reap highest efficiency. Even if the exter-
with lower overpotential, displayed as the yellow line in nal electrical energy was utilized for heating the cell, this
–
H+ H2/H2O AM 1.5
~nc
Global Tilt Flux
e– Vph1 1.23 V dNphdλ (a.u.)
ECB 4
O2 3
NiBi
hν > 1.8 eV
NiMoZn
V 2
EF ph2 h+ ~na
EVB
H2O/O2 H2O
Potential (V)
eV
hν < 1.8 eV e–
+ p
h
p n
n
Metal Anode 1
+
Si Epoxy Au Transparent Transparent
Wafer Contact Graded Tunnel
Handle Reflector Buffer Junction
(a) (b)
+ –
CPV Modules
O2
H2
OH– Electrical Connection
OER HER
H2O Electrochemical Cells
(c) (d)
Figure 3. A PV-EC system developed by various research groups. (a) A PV-PEC cell system developed by the NREL (Young et al. 2017). (Image courtesy of Nature.) (b) The artificial leaf suggested by Har-
vard University (Cox et al. 2011, Noorden 2011). (Photo courtesy of the National Academy of Science.) (c) An organic/inorganic perovskite solar cell-based PV-EC system suggested by the Gratzel group
(Luo et al. 2014). (Image courtesy of Science.) (d) A PV-EC system constructed by a light concentrator, multijunction PV, and membrane electrode assembly-based EC system (Nakamura et al. 2015).
23
research shows the possibility of ultraefficient solar-H 2 er can provide the MPPT technique to follow the maxi-
conversion system. mum power of solar light.
There are several related reports on utilizing converted
The Disadvantages of PV-EC technology for solar light H 2 conversion. The Garrigos
Systems Without Converters group suggested the insulating-type topology of the con-
The conventional PV-EC systems without converters have verter to scale up the PV-EC system, which is caused by
clear disadvantages, e.g., they are best-performed with high voltage generated from the PV. The same group pro-
specific light conditions. If the light density varies, as the posed the topology to precisely regulate the output current
real sunlight intensity changes every hour, the I-V charac- control region, as shown in Figure 4(a). This situation only
teristics of a PV varies, so it is difficult to predict and opti- occurs when the EC needs more voltage than the VPV,max,
mize the best performing condition. For practical which requires delicate duty control. With the Agbossou
utilization, the PV-EC system should be flexible regardless group, the design principle of a converter covered the
of sunlight. To maximize PPV,max and to keep track of the whole H 2 generation and the H 2 storage system.
intensity of sunlight, there is no reason to postpone the The Nam and Ha group reported the casual relation
power converting technique. Therefore, the dc–dc convert- between the converter on/off ratio, the duty and final
Output Capacitor
EC
4–20 mA and Converter
Telemetry
uC
Error
Amplifiers
Input Capacitor
PV
(a) (b)
Figure 4. The various analyses of a converter-assisted PV-EC system. (a) The topology of the converter for output current control when the
EC cannot properly manage the power from a PV (Garrigós et al. 2014). (Photo courtesy of Elsevier.) (b) A converter efficiency measurement
system based on the ratio between input and output electrical power (Chang et al. 2017). (Photo courtesy of the American Chemical Society.)
uC: microcontroller.
25 1.0
U. Tokyo EPFL, STH 12.3%
Tandem PV U. Osaka, STH 2.93%
Single-Junction PV U. Monash
SNU, STH 20.6%
Reported STH Efficiency (%)
15 0.6
NREL EPFL
Caltech
10 Uppsala 0.4
U. Hawaii NREL MIT
GM
Texas A&M
5 UC Berkeley 0.2
U. Osaka
Figure 5. The reported efficiency of a PV-EC system: (a) the reported STH efficiency of a PV-EC system by year and (b) the PH2 /PPV,max (produced
H2 energy compared to the solar-driven maximum electrical power) value based on a surface-area ratio between EC and PV. A high PH2 /PPV,max with
a low A EC /A PV indicates an economical PV-EC configuration. EPFL: École Polytechnique Fédérale de Lausanne; NREL: National Renewable
Research Laboratory; SNU: Seoul National University.
he fuel-cell (FC) concept was invented technology. The Government of India promotes various
T
and demonstrated in the early 18th centu- schemes and policies for research and development by
ry by Humphrey Davy. The FC itself was the country’s major FC system players, including research
developed in 1839 by the chemist William and educational institutions and industries.
Grove, who conducted a series of experi-
ments with what he called a gas-voltaic battery. The term Classifications of Conventional FCs
fuel cell was first used in 1889 by Charles Langer and Lud- An FC is the main energy source of modern electric vehi-
wig Mond, who researched FCs using coal gas as a fuel. In cles (EVs) such as PEMFC EVs, which will likely become
the early 1960s, the National Aeronautics and Space more common due to their zero-emission advantages and
Administration and its industrial partners conducted the other beneficial uses in the transportation sector and
experiments on manned space vehicles based on alkaline as distributed storage when used with advanced converter
FCs (AFCs). Later, the international FC made advances in and battery technologies in the smart grid. Figure 1 pro-
the AFC for the Apollo space mission, which resulted in vides a description and operation of each class of FC cate-
supporting the requirements of drinking water and elec- gorized on the basis of the fuel used in the fuel reformer.
tricity for the astronauts.
Government policies in India have helped promote Direct-Methanol FCs
clean transportation and the development of proton- The direct-methanol FC (DMFC) is a relatively new type. It
exchange membrane FC (PEMFC) vehicles in automotive resembles a PEMFC in that it uses polymer electrolyte (sul-
applications. In 2004, Banaras Hindu University (BHU) and fophynelated sulfonic) as an electrolyte. A typical solitary
the Ministry of New Renewable Energy developed a DMFC can supply just 0.3–0.5 V under loaded conditions.
motorcycle using new FC technology based on PEMFCs. In DMFCs are used to replace the batteries for cameras,
the 2010s, the Indian Space Research Organization and scratch-pad personal computers, and other convenient
TATA Corporation Ltd. jointly developed the passenger electronic applications within the power range of 1 W–
vehicle project named “Starbus” based on the PEMFC 1 kW. The internal operation is constrained by two vital
processes, which lower the framework efficiency (40%).
The principle of operation of the DMFC on the basis of
Digital Object Identifier 10.1109/MELE.2017.2784633
Date of publication: 28 February 2018 chemical equations is shown in Figure 2.
Compressed Water
Air (H2O)
Heat
2–
Appliance
H2O
CGDL
Field Plates
Fuel: Hydrogen
Efficiency: 50%
Name: PEMFC
(CCC)
2–
H+ MEA
e– H2
ACC
AGDL
Bipolar Plates
Figure 1. A description of the operation of an FC with a representation of the characteristics of major FC types based on the use of a
membrane electrode assembly. AGDL: anode gas diffusion layer; ACC: anode carbon catalyst; MEA: membrane electrode assembly;
CCC: cathode carbon catalyst; CGDL: cathode gas diffusion layer.
Electron Flow
Methonal Oxygen
Hydrogen Ions
CGDL
AGDL
Carbon
Dioxide Bipolar Plates AGDL Plus Electrolyte CGDL Plus Bipolar Plates Water
(Polymer/Graphite Anode Catalyst (Sulfophynelated Cathode Catalyst (Polymer/Graphite
Composite) (Platinum Alloy) Polysulfonic) (Platinum Alloy) Composite)
Electron Flow
Hydrogen Oxygen
Hydrogen Ions
CGDL
AGDL
Excess Bipolar Plates AGDL Plus Electrolyte CGDL Plus Bipolar Plates Water
Hydrogen (Platinum/Graphite Anode Catalyst (Polystyrene Cathode Catalyst (Platinum/Graphite
Composite) (Platinum) Sulphonic Acid) (Platinum) Composite)
Hydrogen Oxygen
Hydrogen Ions
CGDL
AGDL
Water Bipolar Plates AGDL Plus Electrolyte CGDL Plus Bipolar Plates Excess
(Metallic Plates) Anode Catalyst (KOH) Cathode Catalyst (Metallic Plates) Oxygen
(Nikhel or Silver) (Nikhel or Silver)
Electron Flow
Hydrogen Oxygen
Hydrogen Ions
CGDL
AGDL
Excess Bipolar Plates AGDL Plus Electrolyte (Liquid CGDL Plus Bipolar Plates Water
Hydrogen (Metallic Plates) Anode Catalyst Phospheric Cathode Catalyst (Metallic Plates)
(Platinum) Acid) (Platinum)
Electron Flow
Syngas
(Hydrogen and Carbon
Monoxide) Oxygen
Carbon Dioxide
Oxygen Ions
CGDL
AGDL
Carbon Bipolar Plates AGDL Plus Electrolyte CGDL Plus Bipolar Plates Carbon
Dioxide and (Metallic Plates) Anode Catalyst (Sodium Cathode Catalyst (Metallic Plates) Dioxide and
Water Carbonate) Oxygen
Electron Flow
Syngas
(Hydrogen and Carbon
Monoxide) Oxygen
Oxygen Ions
CGDL
AGDL
Carbon Bipolar Plates AGDL Plus Electrolyte CGDL Plus Bipolar Plates Excess
Dioxide and (Metalic Plates) Anode Catalyst (Ceramic) Cathode Catalyst (Metalic Plates) Oxygen
Water
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Topologies Ultra
PGS
CHEV
le Sy
SHEV
ICE n Mach
of Electric ine –
Vehic
Vehicle
Recti Vehicles +
fier SP Gear Inverte
Ve H V Box r
G hic E V P HE Rectifie
r
le tem
ler
Sys L o
Sy le wer
up
hic
ste Ve State
Co
m Chargo f
To e
e
s
ue
G
Ca
sion
rq
ICE
ion
Low
ive
iss
er S
smis
ns
sm
pee
te
an
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ler
-In
Tran
Tr
ine
e
tric
PS
oup
iv
ec
se ns
D
ach
eC
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Ca Inte
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M
nM
-
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gi
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En
G
ve ac
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– Tra
rte
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Bat capacito
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or
dc/arter
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tte
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nk
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ill d
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S
Figure 8. A description of the topologies of drivetrains for EVs in India. FCHEV: FC hybrid EV; SHEV: series-hybrid EV; PHEV: parallel-hybrid EV;
SPHEV: series-parallel-hybrid EV; CHEV: complex-hybrid EV; BEV: battery EV; RDAB-IBDC: resonant dual-active bridge-isolated bidirectional dc–dc
converter; FCS: FC stack; M: motor; G: generator; PSD: power split device.
Prediction of FC Vehicles
Sales over the World Market (Including India)
400,000
North America
350,000
FC Vehicles (Sales)
Figure 9. A prediction of FC vehicle sales in the world market. (Data taken from Pike Research/Open Energy Information.)
11,200
9,800
FC Vehicles Cost ( /Kwnet)
8,680
8,400 Target by Target by
7,200 the 2020 the 2030
7,000 5,800
5,600 4,560
3,700
4,200 3,100
2,000
2,800 1,800
1,400 1,000
Figure 10. Projected PEMFC system costs in the Indian market. (Data taken from the Center of FC Technology 2017.)
(a) (b)
Figure 11. The breakdown cost of PEMFC components in (a) 2008 and (b) 2016. (Data taken from the Center for FC Technology 2017.)
Fuel Efficiency and Carbon-Dioxide Reduction (%)
EV (BEV or FCV)
Plug-In HEV
Full HEV
Mild HEV
Micro HEV
Figure 12. The different levels of electrification to reach the target set by the 1997 Kyoto protocol in the world market to reduce greenhouse
gases. HEV: hybrid EV. (Data taken from the Ministry of New and Renewable Energy 2016.)
Figure 14. The deployment of hydrogen-fuel stations in the world market, including the Faridabad hydrogen-fueling station. (Data taken from the
National Fuel-Cell Symposium 2016.)
region would have more hydrogen stations compared to and the need of zero-emission vehicles in logistic hubs, as
the rest of the Eurozone as well as the United States, as well as identified specific fuel-supply strategies to meet
shown in Figure 14. the growth of FC technology. Several environmental and
economic drivers are inspiring the FC technology players
Development of FC Vehicles in India in developing countries such as India. PEMFCVs have
There have been a few significant developments for FC many merits compared to ICEs and hybrid vehicles, e.g.,
vehicles in India. they are efficient and produce less or no greenhouse
xxA group of BHU scientists and the Ministry of New gases. According to experts, the future belongs to modern
and Renewable Energy achieved a breakthrough event FC vehicles. Therefore, we believe there is huge potential
in cutting-edge FC vehicle technology. The fuel box for for FC vehicles in India.
a motorcycle weighs roughly 17 kg, or twice that of a
tank with 10 L of petrol. This lasts for 70–80 km before For Further Reading
a recharge is necessary. During tests, the three-wheel- Centre for Fuel Cell Technology. (2017). [Online]. Available:
https://www.arci.res.in/centres-about-fuel-cell-technology
er clocked a range of 50–60 km.
Ministry of New and Renewable Energy. (2016, June).
xxA PEMFC battery hybrid van has been developed. Hydrogen energy and fuel cells in India—A way forward. Gov-
xxA reformer for a 10-kW PEMFC system was developed ernment of India. New Delhi. [Online]. Available: http://mnre
and tested in the CFCT. .gov.in/schemes/new-technologies/hydrogen-energy/report-
xxTATA Corporation Ltd. and the Indian Space Research on-hydrogen-energy-fuel-cells-in-india-way-forward/
Central Electrochemical Research Institute. (2012). Fuel
Organization took the lead role in introducing the lat-
cells: Electrochemical power sources division. [Online]. Avail-
est FC vehicle technology with the new FC-based pas- able: http://www.cecri.res.in/ResearchAreas/Electrochemical-
senger vehicle, “Starbus,” during 2012–2013. PowerSources
National Fuel Cell Symposium. (2016). [Online]. Available:
Comparison http://www.nfcrc.uci.edu/nationalfuelcellsymposium/2016
The drivetrains of EVs are distinguished based on key
parameters such as propulsion, efficiency, refueling Biographies
time, speed (average maximum speed), acceleration Bandi Mallikarjuna Reddy (ree1505@mnnit.ac.in) is with
(average), cost, and technology. Table 1 shows a compar- the Electrical Engineering Department, Motilal Nehru
ison of the various EVs. The drivetrains of FC vehicles National Institute of Technology Allahabad, India.
have excellent advantages and good feasibility that can Paulson Samuel (paul@mnnit.ac.in) is with the Electri-
be implemented if the required technology is achieved cal Engineering Department, Motilal Nehru National Insti-
by 2025 in India. tute of Technology Allahabad, India.
Narapureddy Siva Mohan Reddy (nsiva.fch@iitr.ac.in) is
Conclusions with the Chemical Engineering Department, Indian Insti-
This article explored the Indian PEMFCV vehicle market tute of Technology, Roorkee, Uttarakhad, India.
with respect to the need for FCs in the transportation field
©istockphoto.com/jeremyiswild
The Future Is
Present in California
or years, hydrogen fuel and fuel- these zero-emission vehicles (ZEVs) on the road by the
F
cell electric vehicles (FCEVs) have been early 2020s.
consistently referred to as “five years away More than 30 open fueling stations with full retail oper-
from commercialization,” even among pro- ations serve communities in Los Angeles and Orange
ponents of vehicles powered by alternatives counties, near San Diego, inland to Riverside, and north to
to conventional gasoline. Year after year, commercializa- the San Francisco Bay Area and Sacramento region. North-
tion seemed just out of reach. Critical FC technology south travel between these markets is made possible by a
advancements took longer than expected; hydrogen stor- station located on the property of Harris Ranch, shown in
age, compression, and dispensing standards needed more Figure 1, a landmark in the city of Coalinga. Owing to the
fine-tuning; and favorable business opportunities for fuel- vehicles’ range and rapid fueling capability and in combi-
ing infrastructure came a bit slower. Today, in California, nation with strategically sited fueling stations, today’s Cal-
that is no longer the case. ifornia FCEV drivers can travel to northern Tahoe and
There is widespread agreement among auto manufac- Santa Barbara. Moreover, California is currently on track to
turers and other light-duty hydrogen transportation stake- develop a fueling infrastructure capable of supporting at
holders that the technology has successfully transitioned least 25,000 vehicles by 2020.
from the precommercial to early-commercial market The transition from a perpetual promise to today’s
phase. At least three different models of early-market reality was made possible in California by dedicating time
FCEVs are available for lease or purchase across the state. and resources to supporting FCEV deployment and devel-
As of October 2017, nearly 2,500 FCEVs have been regis- oping hydrogen fueling infrastructure. Without a doubt,
tered with the state’s Department of Motor Vehicles (DMV), hydrogen as a transportation fuel has arrived, and there
and the latest projections estimate tens of thousands of are several efforts underway to ensure that the last few
years’ momentum is not only maintained but also accel-
erated in the near future. An examination of the timeline
Digital Object Identifier 10.1109/MELE.2017.2784634
Date of publication: 28 February 2018 (see “Hydrogen in California”) of fueling infrastructure
1961
First Automotive Emissions Regulations
in Nation by California Bureau of Air Sanitation
2018–2025
California Fuel-Cell
Partnership Publishes a
2013
California Roadmap
Hyundai Tucson Fuel (2013–2023)
Cell: First Mass-Produced Assembly Bill 8:
FCEV Extends AB 118 with
2014
California Status: 30+ Retail Fueling Stations Open, 30+ Additional Stations Funded,
2017
does not require any change in owners’ driving, fueling, or prospective methods have been introduced, including
ownership habits. A ZEV with these characteristics offers a some with negative carbon intensities where the hydrogen
heightened ease of adoption and can make the vehicle an production process sequesters GHGs that would otherwise
attractive choice. These goals help ensure accelerated be emitted by the feedstock fuel.
growth of zero-emission transportation once the neces- Although this ZEV regulation established commitment
sary fueling infrastructure and vehicle supply chains have and criteria for ZEV targets, experience gained during its
been established. decades-long implementation has emphasized that this is
Hydrogen offers great flexibility in the utilization of only one of several initiatives necessary to ensure the suc-
resources, including renewable energy sources available to cessful market launch of new vehicle motive technologies.
California and to the country at large. Since the passing of The development of fueling infrastructure represents a
the state’s ZEV regulation, a wide array of production meth- second major aspect that requires a similar commitment,
ods have been studied, including steam-methane reforma- concurrent with efforts for the deployment of ZEV tech-
tion, electrolysis (powered either by the grid or dedicated nologies. This is true of all alternative vehicle fuel options.
renewable resources), and tri-generation, i.e., the coproduc- Additional critical aspects for the successful market
tion of hydrogen, electricity, and heat from the integration launch of ZEVs include public outreach and awareness,
of a specially designed FC system with biogas resources at consumer incentives, education for planning authorities
municipal waste treatment or similar facilities. Additional and emergency responders, and so on.
16
16
16
16
17
17
17
gasoline fueling.
20
20
20
20
20
20
20
20
This type of retail experience
4,
1,
2,
3,
4,
1,
2,
3,
Q
Q
has been pioneered in the past
Figure 6. A representation of the growth in retail hydrogen sales and FCEV deployments in Califor- few years within California’s fuel-
nia. Q: quarter. (Image courtesy of Andrew Martinez.) ing network. This has not been a
trivial matter, and significant
of the state’s hydrogen fueling network. A critical first-hand knowledge has been gained through the
aspect of the fueling network developed in California experience of California’s efforts. One early example
is the emphasis on a familiar, reliable retail fuel sales came in 2015, when the station on the California State
environment. As previously mentioned, the ultimate University, Los Angeles (CSULA) campus became the
goal for hydrogen fueling network development is to first in the world to demonstrate hydrogen metering
provide a seamless transition from conventional gas- accuracy at tolerances sufficient to enable retail sales.
powered vehicles to zero-emission FCEVs. This tran- Accurate metering is a fundamental principle of retail
sition requires not only vehicles that provide the sales, as it provides reassurance to customers that they
same capabilities, e.g., expected range, performance, are properly billed, as well as to station operators that
seating capacity, and storage capacity, but also fuel- they are receiving proper revenue for the true amount
ing options that provide service comparable to that of hydrogen sold.
of gas stations. The CSULA station demonstrated sufficient metering
Today, all stations funded in California are required accuracy according to a set of standards developed and
to provide this familiar retail fueling experience. adopted first in California by the Department of Food and
Agriculture’s Division of Measure-
ment Standards (DMS). Later that
same year, the West Sacramento
Air Compressor and Water Chiller
(Behind Convenience Store) fueling station became the first in
Compressor High Pressure the state to officially achieve fully
Hydrogen retail operations. These successes
Storage
were possible because collabora-
Gas tive efforts between the DMS, other
Panel
Hydrogen Chiller state agencies, and industry part-
and Cooling Block Hydrogen ners recognized that existing
Dispenser
national standards were too strin-
gent for available technology.
Tube Trailer
Without modification, national
(Bulk Low-Pressure
Hydrogen Storage) standards could have prevented
Underground retail sales for a number of years
Hydrogen Piping until significant technology de
velopment took place. The DMS,
therefore, instituted a set of revised
standards allowing for looser
tolerances in the near term with
Figure 7. The major components and layout of a conventional hydrogen fueling station with gas-
eous delivery. (Image courtesy of Sandia National Laboratories, adapted from E. S. Hecht and J. specific sunset dates, such that
Pratt 2017.) the metering technology would
Obstacles to the
Success of Fuel-Cell
Electric Vehicles ©istockphoto.com/milehightraveler
Clean Mobility
Green Energy System
Hybrid System
Electrification/
Efficiency Regeneration
Technologies FCEV
Hydrogen
ICE Improvement/
Fuel Cell
CO2 Reduction
PHEV
Plug-In Hybrid
Gasoline
EV
Figure 1. A strategy to develop ecofriendly vehicles. PHEV: plug-in hybrid electric vehicle; HEV: hybrid electric vehicle; ICE: internal combustion
engine. (Image courtesy of Hyundai Motor Company.)
Bipolar Plate
GDL
MEA
y
tricit
Elec
Water
Oxygen
Hydrogen
ton
Pro
(a) (b)
Figure 2. The schematic of (a) a fuel-cell stack of (b) serially connected unit fuel cells.
Figure 6. A crash test performed on an FCEV: (a) a view from the side and (b) a view from the bottom. (Images courtesy of Hyundai Motor Company.)
The Island
Hydrogen Project
n 2014, the transport sector was refueling stations are needed to decarbonize the trans-
I
responsible for 23% of total greenhouse port sector. This article describes the Island Hydro-
gas emissions in the European Union (EU). gen project, which introduced and tested new solutions
During the same year, 13% of that sector’s to produce and use hydrogen as a fuel for vehicles
emissions came from the maritime seg- and vessels.
ment, a number that is expected to rise during the com- Worldwide, the primary companies in the automotive
ing years. The transport sector’s share of renewable industry have already developed fuel-cell electric vehi-
energy in 2014 was just 5.9%, mostly comprising biodies- cles (FCEV). Major improvements from one generation to
el and bioethanol fuel. When we compare this to electric- the next have resulted in hydrogen vehicles with range
ity generated in the EU from renewable sources, at 25.4%, and reliability parameters comparable to conventional
it is clear that electricity generation is leading by a sig- vehicles. The basic principle of an FC is that hydrogen
nificant margin. Electrification is a solution that will help combines with the oxygen from air in the FC stack and
reduce the transport sector’s reliance on hydrocarbon- produces an electric current, which then powers the
based fuels. New energy infrastructures such as hydrogen electric motors. The short-term energy balance between
the FC and the electric motors is facilitated using a bat-
tery. If the battery capacity is much larger than the FC
Digital Object Identifier 10.1109/MELE.2017.2784636
Date of publication: 28 February 2018 capacity, then the FC has the role of extending the range
Trial Outcomes
A measurement campaign at the
vehicle refueling station lasted four
months and was completed in
April 2016. Figure 3(a) shows the
distribution of the refill events Hydrogen Fuel-
according to the mass transferred Cell Vehicle Compressor Buffer
during the refill. The average mass
Figure 2. An M1 hydrogen refueling station in the United Kingdom. (Photo courtesy of ITM Power.)
transferred was 1.355 kg H2, which
is the equivalent of 45.12 kWh
(lower heating value). In the larger,
similar trial completed by the U.S. Mass Refilled Time to Refill
National Renewable Energy Labora- 12 15
Refill
tory (NREL), a value of 2.13 kg was 10
Instances
Refill Instances
Refill Instances
reported (NREL 2011). The Island 8 10
Hydrogen value was influenced by
6
the refueling of Microcabs, pro-
duced by a U.K.-based manufactur- 4 5
er, with a tank capacity of 1.8 kg, 2
which is significantly smaller than 0 0
other FCEVs such as the ones used 0 0.5 1 1.5 2 2.5 3 3.5 0 1 2 3 4 5 6
in the NREL trial. Mass (kg) Time (min)
Figure 3(b) shows the distribu- (a) (b)
tion of the refill events according
to the time taken for each refill. Figure 3. The frequency of refueling events versus (a) the mass of hydrogen gas dispensed and
(b) the time for refill.
The average time for refill was
2 min, 55 s. The refueling time
reported by NREL was 3 min, 26 s. By dividing the energy
of the mass refilled by the time taken to refill, we calcu- Mass Refilled Versus Time to Refill
lated that, on average, the FCEVs were charging at a rate 6
of 1 mW of electric power. The correlation between the
mass of hydrogen gas with which the vehicles were 5
refueled and the time needed for refueling is shown in
Minute Refill (min)
4
Figure 4. The relation was not linear because there were
many factors influencing the time to refill, including the
3
outside temperature, the pressure inside the vehicle
tank, and the storage pressure in the station refueling.
2
Site 0
The trial site for the marine hydrogen refill station was Vent- 0 0.5 1 1.5 2 2.5 3 3.5
nor, Isle of Wight, United Kingdom. Figure 5 shows the main Mass Fill (kg)
components of the trial. An ITM Power manufactured elec-
trolyzer with a capacity of 15 kg H2/d was installed. Figure 4. The relation between the refill time and the dispensed mass.
Installation Considerations
Hydrogen Boat A number of factors were consid-
with Internal ered before the electrolyzer could be
Electrolyzer Combustion
Container installed at Baglan to allow for the
Engine
safe operation of hydrogen systems.
The lab at the Baglan Hydrogen
Centre was naturally ventilated,
allowing more than 12 air changes
per hour, meaning that tempera-
Buffer tures inside the lab were similar to
Compressor those outside. This required the
system to be insulated and trace
Cylinders for
Onboard
heated to allow year-round opera-
Hydrogen Storage tion. Figure 7 shows a diagram of
the Hpac40 unit installed at the
Hydrogen Centre. The electrolyzer,
trace heating, and hydrogen com-
pressor can be seen in Figure 7. A
Figure 5. The Isle of Wight marine filling station. (Photo courtesy of ITM Power.) hazard and operability study was
H2 IC Vehicle
Low-Pressure H2 Storage
H2/CH4 Vehicle
CH4 Storage
Compression CH4 and
Electrolyzer
Low Stage and Mixture
High Stage Dispenser
2 × PV power
150
period, i.e., 10–15 December 2013. The system consistently
operated at roughly 85 V with a hydrogen pressure of
14 bar and the stack current fluctuating between 100 and
120 A. Any fluctuations in the stack voltage lead to exag- 100 40
gerated fluctuations in the stack current due to the shape
of the electrolyzer I-V curve.
When not in hydrogen-generation mode, the electro- 50 20
lyzer maintained a small voltage and current to ensure it
was not damaged by low temperatures, a process called
the frost-protection mode. Figure 9 shows the electrolyzer
0 0
operating in this mode on 4 November 2013. A nominal 10 11 12 13 14 15
voltage of 0.8 V is maintained until the stack temperature Time (date)
falls close to 5 °C. When the stack temperature falls to
Stack Current Ambient Temperature
5 °C, the voltage increases to raise the stack temperature. Stack Voltage Stack Temperature
The trial demonstrated the electrolyzer’s ability to gener- H2 Pressure
ate hydrogen year round and for prolonged periods. Oper-
ational data were shared with the Island Hydrogen Figure 8. HPac40 in hydrogen-generation 10–15 December 2013.
1 18
content/ipc/uploads/projects/EN010032/EN010032-001550-
0.95 16 6.1.30%20Carbon%20Lifecycle%20and%20Balance.pdf
0.9 14 Fueling Protocols for Light Duty Gaseous Hydrogen Surface Vehi-
0.85 12 cles, Fuel Cell Standards Committee, SAE International Stan-
dard J2601_201612, 2016.
0.8 10
0.75 8
0.7 6 Biographies
0.65 4 Silviu Nistor (silviu@yurbs.org) is with YoUrban Innova-
00:00 06:00 12:00 18:00 00:00
tions Ltd., Bristol, United Kingdom.
Time (Hours and Minutes)
Stephen Carr (stephen.carr@southwales.ac.uk) is with
Stack Voltage Ambient Temperature the University of South Wales, Pontypridd, United Kingdom.
Air Temperature Stack Temperature
Mahesh Sooriyabandara (mahesh@toshba-trel.com) is
with Toshiba Research Laboratory, Bristol, United K
ingdom.
Figure 9. HPaC40 in frost-protection mode on 4 November 2013.
2018 3 –7 JUNE
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Date of publication: 28 February 2018 .epe2018.com/
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