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Madhuparna Karmakar1, 2
1
Harish chandra research institute, Chhatnag road, Jhunsi, Allahabad-211019, India, and
Homi Bhabha National Institute, Training School Complex, Anushakti Nagar, Mumbai 400085, India.
2
Department of Physics, Indian Institute of technology Madras, Chennai-600036, India.
(Dated: November 16, 2017)
We study the mass imbalanced Fermi-Fermi mixture within the framework of a two-dimensional lattice
fermion model. Based on the thermodynamic and species dependent quasiparticle behavior we map out the
finite temperature phase diagram of this system and show that unlike the balanced Fermi superfluid there are
now two different pseudogap regimes as PG-I and PG-II. While within the PG-I regime both the fermionic
species are pseudogapped, PG-II corresponds to the regime where pseudogap feature survives only in the light
arXiv:1711.05706v1 [cond-mat.str-el] 15 Nov 2017
species. We believe that the single particle spectral features that we discuss in this paper are observable through
the species resolved radio frequency spectroscopy and momentum resolved photo emission spectroscopy mea-
surements on systems such as, 6Li -40K mixture. We further investigate the interplay between the population and
mass imbalances and report that at a fixed population imbalance the BCS-BEC crossover in a Fermi-Fermi mix-
ture would require a critical interaction (Uc ), for the realization of the homogeneous superfluid state. The effect
of imbalance in mass on the exotic Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superfluid phase has been probed
in detail in terms of the thermodynamic and fermionic behavior of this phase. It has been observed that in spite
of the s-wave symmetry of the pairing field a nodal superfluid gap is realized in the LO regime. Our results on
the various thermal scales and regimes are expected to serve as benchmarks for the experimental observations
on 6Li -40K mixture.
E/N
overestimates the ground state energy of the system. The ef-
fect is likely to be more severe at finite temperature where
crucial amplitude and phase fluctuations are neglected within 1.4
a mean field scheme.
An estimate of the inadequacy of mean field approach to
the problem at finite temperature can be made from the fact 1.6
that mean field theory overestimates the T c scales by a fac-
tor of more than 4 both in case of balanced [7075] as well
population imbalanced Fermi superfluids [51]. This is a cru- 0 0.5 1.0 1.5 2.0
cial observation owing to the fact that many of the predictions 0
for imbalanced Fermi superfluids are being made based on the
mean field theory.
FIG. 1. Color online: Variation of free energy density with pairing
While there is now a consensus about the thermal behav- field amplitude at different mass imbalance ratio. The population
ior of balanced Fermi superfluid [76, 77], the same can not imbalance is set to zero.
be said about the Fermi-Fermi mixture. Within the purview
of lattice fermions, there is certainly a void in our present un-
derstanding of such mixtures, specially at finite temperatures. species is pseudogapped upto T58.5nK, while in the
On the other hand, a lattice fermion model is a suitable choice light species the pseudogap survives upto T > 108nK.
keeping in view the optical lattice experiments that are carried
out on ultracold Fermi gases. What is the Tc scale of a mixture In presence of population imbalance, homogeneous su-
such as 6Li -40K ? How does such a system behave across the perfluid state (with zero momentum pairing) is realized
BCS-BEC crossover and most importantly how does the pseu- only beyond a critical interaction Uc . This is in remark-
dogap physics play out in the back ground of an imbalance of able contrast to the balanced case where any arbitrarily
fermionic masses in the system? While an experimental inves- small attractive interaction gives rise to a stable homo-
tigation to answer such questions is awaited, one can certainly geneous superfluid.
make theoretical predictions.
Imbalance in population leaves its imprint on the su-
Motivated by these questions, in this paper we present a
perfluid gap. In spite of an isotropic s-wave interaction
detail finite temperature analysis of mass imbalanced Fermi
finite momentum scattering gives rise to nodal super-
mixture within the framework of lattice fermions. We use a
fluid gap.
numerical technique which takes into account the phase fluc-
tuations of the ordering field and can access the thermal tran- Rest of the paper is organized as follows. In section II we
sitions with quantitative correctness. Apart from investigating discuss about the model and the numerical method that has
the behavior of mass imbalanced system across the BCS-BEC been used to study the imbalanced Fermi mixture. Section III
crossover we also investigate the interplay of mass and pop- discusses our results for population balanced and imbalanced
ulation imbalances. Before making quantitative predictions systems with imbalance in mass. We further present quan-
about the 6Li -40K mixture we have discussed how the exotic titative estimates of the thermal scales corresponding to the
Fulde-Ferrell-Larkin- Ovchinnikov (FFLO) superfluid phase 6Li -40K mixture. We touch upon certain computational issues
reacts to the imbalance in mass in terms of their thermody- in the discussion section IV and conclude with section V.
namic and quasiparticle behavior. We highlight our principal
observations below before proceeding to discuss the numeri-
cal technique and the results obtained from the same. II. MODEL, METHOD AND INDICATORS
6 6 tem. With h being set to zero we use the mass imbalance ratio
as the tuning parameter to investigate the various proper-
2 2 ties. We map out the ground state phase diagram based on the
5 5 variational mean field calculation (discussed in the previous
1 section) and in Fig.1 show the dependence of free energy on
4 1 40.1 0.3 0.5 0.7 0.9
the pairing field amplitude 0 and mass imbalance ratio for
0.1 0.3 0.5 0.7 0.9
the selected interaction strength U=4tL . The ground state en-
ergy shows a single minima and correspond to a homogeneous
superfluid state with the pairing field amplitude (0 ) being al-
most independent of the choice of the mass imbalance ratio.
FIG. 2. Color online: Ground state (a) pairing field amplitude and Both the pairing field amplitude as well as the superfluid gap
(b)superfluid gap in the -U plane for the population balanced sys- at the Fermi level increases monotonically with U. We show
tem. Strong interaction and small mass imbalance ( 1) leads to a these behavior in the -U plane in Fig.2a and 2b, respectively.
larger pairing field amplitude and gap at the Fermi level. The effect of mass imbalance on the quasiparticle disper-
sion spectra is probed next and we show the corresponding
X spectral function A(k, ) at different mass imbalance ratio in
(q) = i j eiq.(ri r j ) , where, i j = hciH ciL ihc jL c jH i Fig.3. The k-summed quantity of the spectral function corre-
ij spond to the electronic density of states (DOS) and we show
A (k, ) = (1/)ImG (k, ) the species resolved variant of the same (N ()) as the last
A (k, 0) = (1/)ImG(k,
X 0) two panels of Fig.3. For the computation of both the spec-
NL () = h(1/N) | un | ( En )i
i 2 tral function and the DOS we have used the Greens function
Xi,n formalism which gives access to large system sizes and thus
NH () = h(1/N) | vin |2 ( + En )i makes the van Hove singularities prominent. Details on the
i,n Greens function formalism are discusses in section IV.
We observe that at large imbalance in mass there are essen-
tially four branches in the dispersion spectra. Both above and
Here, G (k, ) = lim0G (k, in ) |in +i where below the Fermi level the branches intersect each other at k
G (k, in ) is the imaginary frequency transform of = /2, which gives rise to additional singularities in the form
hck ()ck (0)i. uin and vin are the BdG eigenvectors cor- of subgap and supergap states in the DOS. However, there is
responding to the eigen values En for the configurations under no spectral weight at the Fermi level which ensure that the
consideration. N = L2 is the number of lattice sites. underlying ordered state is gapped across the range of . In a
later section we would find that this behavior is remarkably al-
tered once a population imbalance in introduced in the system.
With decreasing mass imbalance the branches merge together,
III. RESULTS leading to the well known two-branched BCS spectra as
1 [93].
In agreement with the behavior of the spectral function we
In this section we discuss the results obtained through our observe that for the system at or close to the mass balanced
numerical simulations. We categorize our observations in two situation, the species resolved DOS exhibits prominent hard
groups viz. (i) mass imbalanced Fermi-Fermi mixture with gap at the Fermi level separated by the characteristic BCS-like
balanced population and (ii) mass imbalanced Fermi-Fermi coherence peaks. Increasing imbalance gives rise to subgap
mixture in presence of population imbalance. Within each and supergap states.
category we discuss the ground state and finite temperature
behavior separately.
2. Finite temperature
NH (!)
NL (!)
0.4
1
0.2
0 0
3 2 1 0 1 2 3 3 2 1 0 1 2 3
! !
FIG. 3. Color online: Ground state dispersion spectra at different mass imbalance ratio . The last two panels show the dependence of the
density of states (DOS) for the (a) light and (b) heavy fermion species. Note the sub and super gap features in the DOS at large mass imbalance
ratio.
a finite peak at q = 0. Based on these two quantities we map the fermionic properties such as single particle DOS, spectral
out the mass imbalance-temperature (-T) phase diagram at function etc. (discussed later) shows us how the information
U=4tL and show it in Fig.4a. Note that in a two-dimensional about the quasiparticle behavior significantly alters the phase
system such as the present one, thermal transitions are pos- diagram in Fig.4a.
sible only through a Berezinskii-Kosterlitz- Thouless (BKT) In Fig.4c we show the BCS-BEC crossover at a selected
transition. The Tc scales discussed here correspond to the mass imbalance ratio of = 0.15, corresponding to the experi-
BKT transition temperature. mentally realized Fermi-Fermi mixture of 6Li -40K [18, 19, 21,
There are two thermal scales in this phase diagram viz. Tc 22]. Further, we compare our result with the one obtained for
and T which demarcates the phases as superfluid, pseudogap a mass balanced system, so as to demonstrate the suppression
and normal. While Tc corresponds to the temperature beyond of Tc by imbalance in mass.
which the long range phase coherence in the pairing field is Across the BCS-BEC crossover the behavior of the Tc scale
lost, T marks the loss of short range pair correlations leading is governed by different mechanisms at different coupling
to the disappearance of superfluidity. regimes. In the weak coupling regime the thermal scale is de-
Thermal fluctuations are progressively detrimental with in- termined by the vanishing of the pairing amplitude (hhciL ciH ii)
creasing mass imbalance in the system, leading to suppres- as kB T tet/U . At strong interactions where the system com-
sion in Tc as shown in Fig.4a. The observation suggests that prises of molecular pairs the thermal scale is dictated by the
even though at the ground state there is a large pairing field phase correlation of the local order parameter and behaves as
amplitude the state is fragile towards thermal fluctuations and kB T f (n)t2 /U, where f (n) is a function of number density.
rapidly looses phase coherence. The thermal scales Tc and T In Fig.4d we show the composite thermodynamic phase di-
are determined from the pairing field structure factor (S (q)) agram in the -U-T space. A large imbalance in mass sup-
shown in Fig.4b. Away from the weak coupling regime the presses the Tc scale irrespective of the choice of U. For eg., at
short range pair correlations survive upto temperatures T >> U=4tL , Tc 0.16tL at = 0.9, and progressively reduces to Tc
Tc . In the limit of 1 we find T 2Tc . The pseudogap 0.13tL at = 0.5 and to Tc 0.04tL at = 0.1, respectively.
regime is determined based on the temperature dependence of The BCS-BEC crossover remains roughly unaffected (except
the structure factor and pair correlation peak at q = 0 and for this suppression) by the change in the mass imbalance ra-
T correspond to the temperature at which there is no dis- tio, with Uc 5tL corresponding to unitarity with maximum
tinguishable peak in the S(q) and (q) at q = 0. Within Tc [77]. We would come back to the concept of unitarity in a
the pseudogap regime, short range pair correlations survive lattice fermion model in the discussion section of this paper.
in both the fermionic species. Fig.4a is one of the impor- The quasiparticle behavior is discussed next and in Fig.5 we
tant results of this work. It shows how the consideration of show the effect of mass imbalance on species resolved DOS.
phase fluctuations in the numerical framework is important to The effect of mass imbalance on the DOS can be observed
capture the true thermal scales of the mass imbalanced super- through multiple features. A quick look at the magnitude of
fluid system. A finite temperature mean field theory (MFT) the coherence peaks of the DOS in Fig.5 shows that the heavy
can track only T and thus lead to significant overestimation fermion species has its coherence peaks significantly larger
of Tc . However, even though the thermodynamic measures in magnitude as compared to its lighter counterpart. In Fig.5
S(q) and (q) are sufficient to quantify the existence of phase we have shown the species resolved DOS corresponding to
coherence in the system, they lack the information about the three different mass imbalance ratio as = 0.2 (panels (a)
quasiparticle behavior of the fermionic species. Analyzing and (d)), = 0.5 (panels (b) and (e)) and = 0.9 (panels (c)
and (f)). While the difference in magnitude of the coherence 0.25
(a) (b) = 0.1
peaks between the two species is maximum at large mass im- Normal Pseudogap = 0.3
balance, it progressively reduces as the system transits to the T 0.8 = 0.5
= 0.7
balanced situation and at = 0.9 they are almost equal, as 0.15
Tc = 0.9
S(0, 0)
expected from the mass balanced situation. Secondly, we ob-
T(tL )
serve that the two species are now being subjected to differ- 0.4
Superfluid
ent scaled temperatures and the heavy species experiences a 0.05
higher temperature as compared to the lighter ones. This is
because the kinetic energy contribution of the two species are 0 0
0 0.2 0.4 0.6 0.8 1 0 0.05 0.10 0.15 0.20 0.25
T(tL )
now different in presence of imbalance in mass. Thus, there
0.20 10
are now two different pseudogap scales in the system and one (c) (d) 0.16
needs species resolved probes such as rf spectroscopy to ac-
0.15
cess them. Finally, at larger imbalance in mass the pseudogap
Tc (tL )
0.12
8
behavior is almost independent of thermal evolution and per-
U(tL )
0.10
sists even at high temperatures. It is only close to the mass bal- 0.08
0.10
NL (!)
0.05 0.01TL
0.05TL
0.10TL
0.15TL
0.20TL
0.25TL
0.30TL
0
3 2 1 0 1 2 3 3 2 1 0 1 2 3 3 2 1 0 1 2 3
! ! !
(d) T = 0.05TH (e) (f)
T = 0.25TH
T = 0.50TH
0.4 T = 0.75TH
T = 1.00TH
T = 1.25TH
NH (!)
T = 1.50TH
0.2
0
3 2 1 0 1 2 33 2 1 0 1 2 33 2 1 0 1 2 3
! ! !
FIG. 5. Color online: Thermal evolution of DOS at the Fermi level for the light ((a)-(c)) and the heavy ((d)-(f)) fermion species for different
mass imbalance ratio of = 0.2 (panel (a) and (d)), = 0.5 (panels (b) and (e)) and = 0.9 (panels (c) and (f)). At large imbalance in mass the
DOS corresponding to the heavy species has coherence peaks with magnitudes significantly larger than its light counterpart. As the system
approaches the mass balanced situation the coherence peaks of the heavy species reduces and for 1 becomes equal to that of the light
species. The DOS and thus the pseudogap scale is almost independent of temperature at large mass imbalance ratio unlike the situation when
1.
FIG. 6. Color online: Thermal evolution of species resolved (light (left) and heavy (right)) spectral function A(k, ) at selected . All
temperatures are measured in terms of tL , where tL =tH /. Since the heavy species experiences a higher scaled temperature (see text) it
undergoes faster thermal disordering.
alized. It was found that rather than transiting to a polarized comprising of coexisting superfluidity and finite polarization,
Fermi liquid phase the system undergoes transition to a mod- a phase which does not have a ground state counterpart [51].
ulated superfluid state with finite momentum (q , 0) pairing, In the next few sections we discuss the effects of the interplay
known as the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state between population and mass imbalances in the system under
[51, 52, 94, 95]. At weak imbalance in population the sys- consideration.
tem undergoes thermal evolution to a breached pair (BP) state
(b) (c)
1.4 (a) PPFL mc2
hc2 0.6 PPFL 0.6 = 0.1
= 0.3
1.2 = 0.5
= 0.6
mc1
m
h(tL )
m
= 0.9
LO LO
1.0 0.4 0.3
hc1
0.8 USF Unstable
0.2 0
0 0.2 0.4 0.6 0.8 1.0 0.2 0.4 0.6 0.8 1.0 0 0.3 0.6 0.9 1.2
h(tL )
FIG. 7. Color online: Ground state phase diagram for the mass imbalanced system as a function of varying population imbalance at U=4tL ,
in the (a) -h and (b) -m plane. Upto a critical field (hc1 ) say, the system is an unpolarized superfluid (USF). A small gives rise to a small
hc1 and beyond 0.5, hc1 becomes independent of the choice of . For the range of field hc1 < h < hc2 a modulated superfluid (LO) phase
is realized for any choice of . hc2 is only weakly dependent on the choice of beyond 0.5. For h > hc2 the ground state of the system
is a partially polarized Fermi liquid (PPFL). In the -m plane the entire USF regime collapses on to the m=0 axis. The ground state is phase
separated in this regime and undergoes first order transition to the LO state beyond a critical mc1 , say. A second order transition from the LO
to the PPFL state takes place at mc2 . Panel (c) shows how the polarization (m) varies with the effective field h at different mass imbalance ratio
. At the critical field hc1 there is a discontinuous transition between the zero and finite polarization state. The transition is only weakly first
order at small mass imbalance (as 1), while a sharp first order transition is realized in presence of large imbalance in mass.
T(tL )
T(tL )
BP
Tc1
0.05 Tc1 0.05 BP Tc1 0.05
BP Tc2 LO Tc2 Unstable Tc2
Unstable Unstable
Unstable LO LO
0 0
0 0.1 0.2 0.3 0.4 0.5 0 0 0.1 0.2 0.3 0.4 0.5 0 0.1 0.2 0.3 0.4 0.5
m m m
FIG. 8. Color online: Polarization-temperature (m-T) phase diagram at selected mass imbalance ratio of = (a)0.2, (b)0.4 and (c)0.6.
The dashed line correspond to T in each panel. There are three broad thermodynamic phases in each case as the (i)breached pair (BP),
(ii)modulated superfluid (LO) and (c)partially polarized superfluid (PPFL). In the regime of weak polarization the system undergoes second
order thermal transition (shown by black solid line) from BP to the pseudogap phase. At intermediate polarization the low temperature phase
separated (unstable) state undergoes a first order thermal transition (shown by the red solid line). The large polarization regime is LO phase
which undergoes a second order thermal transition. The first order transition regime is demarcated by a tricritical Tc1 and a Lifsitz point Tc2 .
A large mass imbalance in the system leads to significant suppression in the Tc and thus the phase coherent superfluid state but gives rise to a
wider pseudogap regime.
2. Finite temperature phase in the -T plane for a particular choice of effective field
h=0.6tL . Apart from the Tc there are additional thermal scales
The thermal evolution of the system is discussed in terms in this phase diagram based on the quasiparticle behavior. We
of m-T phase diagrams shown in Fig.8 for different choices of discuss them below.
mass imbalance ratio . The thermodynamic phases are deter- For a population imbalanced system the species resolved
mined based on the thermal evolution of pairing field structure DOS at the shifted Fermi level ( = h) shows a non mono-
factor S(q) and polarization m(T). The broad thermodynamic tonic behavior [51]. Increasing temperature leads to progres-
phases remain the same irrespective of the choice of , and sive filling up of the gap upto a temperature Tmax . For T >
with increasing imbalance in population the system transits Tmax a non monotonic thermal evolution sets in and there is
through a breached pair (BP), unstable, LO and PPFL phases now depletion of spectral weight at the Fermi surface with
in each case. Also irrespective of the choice of there is a tri- increasing temperature. In presence of strong interaction the
critical point Tc1 and a Lifsitz point Tc2 in the phase diagram. pseudogap continues to survive upto high temperatures but the
While Tc1 corresponds to the point where the order of tran- scale Tmax rapidly collapses with increasing population imbal-
sition changes from second to first within the BP phase, Tc2 ance [51]. Since Tmax survives upto temperatures significantly
marks the transition from the BP to the LO phase. Unlike the higher than the Tc it is more likely to be accessible to the ex-
continuum case [56] the two transitions are well separated in perimental probes.
a lattice model and the separation increases with increasing In presence of mass imbalance the scale Tmax is now de-
H L
mass imbalance. Presence of mass imbalance significantly pendent on the fermion species as Tmax and Tmax , correspond-
L
alters the regime of stability of the different thermodynamic ing to the heavy and light fermion species, respectively. Tmax
H
phases. A larger imbalance in mass leads to stronger sup- and Tmax sets the scale for the regime of species dependent
pression in Tc and thus a progressively smaller BP regime. pseudogap behavior. We show these thermal scales in the -
The pseudogap regime on the other hand increases monotoni- T phase diagram in Fig.9. There are two pseudogap regions
cally with the imbalance in mass, for example, at h=0 the ratio as PG-I and PG-II. While within the PG-I regime both the
T /Tc 3.33 at = 0.2 and reduces to 2.14 and 1.25 at fermion species are pseudogapped, it is only the light species
= 0.4 and 0.6, respectively. which is pseudogapped in the PG-II regime. As 1 both
H L
As discussed in case of the population balanced superfluid the scales Tmax and Tmax collapses into a single one, as ex-
the species resolved DOS continues to have different thermal pected from a mass balanced system.
disordering scales in the BP regime as well, owing to the dif- In the LO phase, mass imbalance gives rise to intriguing
ferent kinetic energy scales of the two species. The underlying features both in the thermal and quasiparticle behavior. For a
superfluid state in this regime is gapped and undergoes ther- particular choice of population imbalance the mass imbalance
mal evolution to pseudogapped phase with increasing temper- ratio dictates the pairing momenta Q. The signature of the
ature. In Fig.9 we show the thermal phase diagram of the BP same can be observed both in the pairing field structure factor
low temperatures. In agreement with the DOS there is no hard
gap at the Fermi level, while soft gaps or depletion of spectral
0.4 weights are observed at the shifted Fermi levels. As in case
THmax PPFL of the BP phase the thermal disordering scales continues to be
T(tL )
species dependent.
Before closing this section we discuss about two quantities
PG II which crucially depends on the imbalance of population and
mass in the system. The first quantity is the momentum re-
0.2
solved occupation of the fermion species n (k), which maps
TLmax out the Fermi surface architecture. In presence of an under-
PG I
Tc lying inhomogeneous pairing field such as the LO superfluid
we expect a non trivial Fermi surface and show the same for
Superfluid two different choices of mass imbalance ratio =0.4 and 0.6,
0 in Fig.13. As in case of DOS the T=0 calculations are car-
0 0.2 0.4 0.6 0.8 1.0 ried out on a larger system size of 6060 using the variational
technique. Apart from the mismatch in size the Fermi sur-
faces now show two-fold symmetry consequent to the uniax-
ial modulation of the pairing field at this particular parameter
FIG. 9. Color online:Mass imbalance-temperature (-T) phase dia- point. Thermal evolution progressively smears out the direc-
gram at fixed population imbalance of h = 0.6tL . Along with the tional asymmetry in the Fermi surface, and at T > 2Tc the
superfluid regime the figure shows the pseudogap regimes based on expected four-fold symmetry is restored. Owing to the asym-
L H
the species resolved DOS. Tmax and Tmax correspond to the scales
metry of the Fermi surface, pairing now essentially takes place
beyond which the pseudogap behavior becomes non monotonic (see
text). PG-I corresponds to the regime where both the light and heavy only at selected Q values [51].
species are pseudogapped, while in the PG-II regime only the light The second quantity of interest is the low energy spectral
species is pseudogapped. weight distribution A(k, 0) which gives information about the
nature of the superfluid gap. In Fig.14 we plot A(k, 0) at =0.4
and 0.6 as it evolves in temperature. A very interesting behav-
(S(q)) as well as in pair correlation (q), both of which shows ior emerges from this figure, wherein in spite of an isotropic
peak at q , 0. We show the thermal evolution of the same in s-wave symmetry of the pairing field, the superfluid gap is
Fig.10 at = 0.6 and a representative population imbalance now nodal, arising purely out of the finite momentum scat-
of h = 1.0tL , corresponding to the LO phase. At this choice of tering that takes place in the LO phase. The gap isotropy is
parameters the underlying LO phase is uniaxially modulated restored at T>2Tc . Momentum resolved photoemission spec-
as can be seen from the two-fold symmetry of S(q) and (q) troscopy is one such experimental tool which can probe the
at the lowest temperature. With Tc 0.01tL we find that the angular dependence of the gap. While the presence of an un-
state undergoes thermal disordering and acquires a four-fold derlying LO phase guarantees a nodal gap structure, the exact
symmetry TTc . Short range LO pair correlations however symmetry of the gap (as well as the Fermi surface) is dictated
continues to survive upto still higher temperatures and van- by the pairing momentum Q and thus by the mass imbalance
ishes only at T>2Tc . ratio . We believe that such nontrivial behavior of the gap
We next show how the finite momentum pairing in the LO would have intriguing signatures in species resolved transport
regime modifies the quasiparticle behavior. As mentioned measurements. We however do not touch upon those issues in
above the DOS at the shifted Fermi level is pseudogapped the present paper.
even at the ground state and contains additional van Hove sin-
gularities. Thermal disordering smears out these singularities.
The exact number and location (energy) of the van Hove sin- C. Effect of interaction
gularities are altered by the choice of . We demonstrate this
behavior in Fig.11 where we show the thermal evolution of In the last few sections we have discussed how the inter-
the species resolved DOS at two different s mentioned in play of mass and population imbalances bring about several
the figure caption. At =0.4 and 0.6, the finite momentum intriguing features in a Fermi-Fermi mixture, at a particular
pairing takes place at Q = (0, ) and (0, /2), respectively. interaction strength. One of the principal advantages of the
At T=0, the DOS is computed using the variational scheme cold atomic gas quantum emulator is the ability to control
on a system size of 60 60. We have further compared our the interaction strength and thus it is of significant interest
ground state results with the one obtained by Greens function to understand how the interplay between the population and
formalism (shown by dotted curve) and have observed quali- mass imbalances alter the well known picture of BCS-BEC
tative agreement between the two. crossover in balanced Fermi gas.
Thermal evolution of the species resolved spectral function In this section we briefly discuss the interplay and present
A (k, ) along the {0, 0} to {, } scan across the Brillouin our observations in terms of the m-T phase diagram at =
zone for two different choices of are shown next, in Fig.12. 0.6 for different choices of interaction strength in Fig.15. The
The multiband nature of the dispersion spectra is evident at phase diagram remains qualitatively the same at other mass
FIG. 10. Color online: Thermal evolution of pairing field structure factor (S(q)) and pair correlation ((q)) at a representative point (h=1.0tL )
in the LO phase for a mass imbalance ratio of =0.6 and interaction U=4tL . The underlying uniaxially modulated LO state is observed through
the finite Q peaks in S(q) and (q), at low temperatures. Fluctuation progressively disorders the system and restore the four-fold symmetry.
However, signatures of short range correlations survive upto T>2Tc (where, Tc 0.01tL ).
0.25
(a) T = 0.000tL
0.6
(b) T = 0.0000tH
imbalance ratio. Fig.15 can roughly be compared with Fig.8
T = 0.001tL T = 0.0025tH
T = 0.005tL
T = 0.010tL
T = 0.0125tH
T = 0.0250tH
and 9 of ref.[56]. In the limit of small polarization the sys-
T = 0.015tL
T = 0.020tL 0.4
T = 0.0375tH
T = 0.0500tH
tem is in the breached pair state comprising of homogeneous
0.15
superfluidity with finite magnetization. Note that we do not
NH (!)
NL (!)
the BP phase. Akin to the continuum case [56] the first order
NL (!)
FIG. 13. Color online: Thermal evolution of single particle occupation for the different species (n (k)), where = L, H; mapping out the
Fermi surface at =0.4 and 0.6 for h=1.0tL . Note the mismatch in size of the Fermi surfaces owing to the imbalance. The T=0 results are once
again obtained using the variational calculation at large system size of L=60. The anisotropy in the Fermi surface architecture arises due to the
modulated underlying state. The isotropy of the Fermi surface is regained at high temperature.
FIG. 14. Color online: Thermal evolution of low energy spectral weight distribution A(k, 0) at the Fermi level =0.4 and 0.6, mapping out the
superconducting gap structure. Note that inspite of an isotropic s-wave pairing field a nodal gap structure is realized at low temperature. At
T2Tc the gap isotropy is restored.
PPFL
0.10 0.10 0.10 PPFL
PPFL
T(tL )
T(tL )
T(tL )
BP Tc1 BP
0.05 0.05 Tc1 0.05
FIG. 15. Color online: Polarization-temperature (m-T) phase diagram for =0.6 at different interactions (a) U=3tL , (b) U=4tL and (c) U=6tL .
At strong interaction (U=6tL ) the system undergoes a second order transition from a BP to LO regime without an intervening unstable regime
involving first order transition. There is only one Lifsitz point Tc2 in this case.
22]. Even though superfluidity is yet to be achieved, Feshbach (USF). The finite temperature counterpart of the same leads to
resonance as well as the formation of heteromolecules 6Li -40K the BP phase. In the weak coupling regime (U< 4tL ) the sys-
has already been attained for this mixture. tem is a partially polarized Fermi liquid (PPFL) in the ground
In order to analyze the behavior of 6Li -40K mixture we state and does not show any long range order.
choose the mass imbalance ratio to be =0.15. For the popula- Fig.16b shows the temperature dependence of polarization
tion imbalance we select h=0.6tL corresponding to the system across the BCS-BEC cross over. Increasing interaction sup-
in BP regime, close to unitarity. We believe that as compared presses the polarization and homogeneous superfluid state is
to the LO superfluid regime the BP phase is more readily ac- realized over a wider regime of temperature. At large inter-
cessible to the experimental probes, owing to its higher ther- actions where the fermions form tightly bound pairs, the re-
mal scales. This justifies our choice of h = 0.6tL . quired population imbalance to break the pair and create finite
We begin the discussion of our results by demonstrating the polarization is large, leading to the suppression in the polar-
BCS-BEC crossover for the 6Li -40K mixture. Fig.16a shows ization. In striking contrast is the weak (U < 4tL ) interaction
the pairing field structure factor (S(0,0)) (at q = 0) across the limit where even at the ground state there is a large finite po-
BCS-BEC cross over. In the intermediate and strong cou- larization, indicating a PPFL state.
pling regime (U 4tL ) the ground state of the system at this We present the Tc scale for the 6Li -40K mixture as deter-
population imbalance correspond to an unpolarized superfluid mined from S(0, 0), in Fig.16c. There are two key effects
T/tL T/tL species at different interactions. At U = 3tL there is no long
0.00 0.02 0.04 0.06 0 0.1 0.2 0.3 range ordered ground state of the system, consequently there
U = 3tL
(a) U = 4tL (b) U = 4tL is no hard gap at the Fermi level even at the lowest tempera-
0.8 U = 5tL U = 5tL 0.4
ture. There is a depletion in spectral weight at the Fermi level,
S(0, 0)
U = 6tL
m(T)
U = 6tL
U = 7tL
U = 7tL U = 8tL
giving rise to a pseudogap phase. Thermal evolution leads
0.4 U = 8tL
0.2 to further depletion of the spectral weight at the Fermi level,
in agreement with m(T ) (Fig.16b) which shows a reduction
in polarization at high temperatures, indicating emergence of
short range correlations. A larger interaction (U = 4tL ) gives
18 rise to a hard gap at the Fermi level, which fills up monoton-
0.04 (c)
(d)
Tc (nK)
ically with temperature before undergoing a non monotonic
Tc (U)/tL
L H
12 thermal evolution at Tmax (Tmax ) corresponding to the light
L H
(heavy) species. At U=5tL the Tmax and Tmax scales are sig-
0.02 6 nificantly high and are not shown in Fig.17.
We next analyze the momentum resolved spectral func-
0 tion A (k, ). In Fig.18 we show the thermal evolution of
3 4 5 6 7 8 3 4 5 6 7 8 the species resolved spectral function at three different inter-
U/tL U/tL
actions, along the {0, 0} to {, } scan across the Brilllouin
zone. The figure shows species dependent thermal scales in
the problem.
FIG. 16. Color online:(a) Pairing field structure factor (S(0, 0)) at a
population imbalance of h = 0.6tL and mass imbalance ratio of = The spectral function for U=3tL reveals that at the lowest
0.15 (corresponding to the 6Li -40K mixture) for different interactions. temperature there is finite weight at the Fermi level and conse-
(b) Temperature dependence of polarization (m(T)) at different inter- quently the dispersion spectra is gapless for both the species.
actions. A large interaction suppresses the polarization. (c) BCS- Increase in temperature leads to depletion of weight, giving
BEC crossover at = 0.15. Tc (U) has its maxima (corresponding rise to a small but finite gap at the Fermi level. This is a
to unitarity) at U = 5tL , (d) BCS-BEC crossover replotted in terms special case of temperature driven gapless to gap transition,
of the experimental scales appropriate for the 6Li -40K mixture. Note arising out of short range correlations.
that at a fixed population imbalance the homogeneous superfluidity
sets in beyond a critical interaction (U > Uc ). The dashed line shows We now present the thermal phase diagram across the BCS-
that for U < Uc the superfluid order vanishes. BEC crossover for the 6Li -40K mixture, in Fig.19a. While in
the PG-I regime both 6Li and 40K would show pseudogap be-
havior, in the PG-II regime it is only the 6Li species which is
in the pseudogap phase. 40K in the PG-II regime is a partially
which decides the behavior of the Tc scale. We discuss them
polarized Fermi liquid. Note that a similar observation has
point- wise. (i) The primary effect is the suppression of the Tc
also been made in the context of continuum model [38, 57].
by the imbalance in mass. Close to unitarity, at U = 4tL the Tc L H
Both Tmax and Tmax are significantly higher than Tc and con-
for a mass balanced system is Tbal c 0.15tL , in comparison to
sequently are better accessible to experimental probes, such
Timb bal
c 0.03tL 0.2Tc for 6Li -40K mixture. The estimated Tc
as rf spectroscopy.
of the 6Li -40K mixture (at U=4tL ) amounts to Timbc 11.7nK.
(ii) The second effect on Tc arises out of the population im- For 6Li -40K mixture close to unitarity we expect the PG-I
L
balance. An weaker interaction shrinks the regime of both regime to survive upto Tmax 58.5nK while the PG-II regime
H
the homogeneous and modulated superfluid and rapidly gives should be observable even at Tmax 108nK, as shown in
way to a PPFL state. Thus, at a fixed population imbalance Fig.19b. Another suitable probe is the momentum resolved
the system can be in a PPFL state at weak interactions, while spectroscopy which can provide evidence of unequal thermal
a large interaction would correspond to a homogeneous su- disordering temperatures corresponding to the two fermion
perfluid state at the same imbalance. Consequently, at a fixed species. A behavior that would be qualitatively similar to the
population imbalance, on traversing through the BCS-BEC one shown in Fig.18.
crossover a homogeneous superfluid state would be realized
only beyond a critical interaction (Uc ). The behavior is sig-
nificant and is in contrast to the balanced system in which any
arbitrarily small attractive interaction gives rise to a homoge- IV. DISCUSSION
neous superfluid state.
Fig.16c further shows that Tc (U) has a peak at U = 5tL , cor- The preceding sections comprise of the main results of this
responding to the unitarity in the context of lattice fermion work. We now touch upon in brief certain aspects on the
model (see discussion section). We estimate the Tc (U) scale model under consideration and its connection to cold atomic
in experimental units and map out the expected BCS-BEC experiments in continuum; we also discuss about the Greens
crossover for the 6Li -40K mixture in Fig.16d. At unitarity the function formalism that has been used in this work to com-
mixture has a Tc 15nK. pute the ground state quasiparticle properties and benchmark
In Fig.17 we show the thermal evolution of DOS for the two the results obtained with those from Monte carlo simulations.
0.15 (a) U = 3tL (b) U = 4tL T = 0.01tL 0.15 T = 0.01tL
T = 0.04tL (c) U = 5tL T = 0.03tL
T = 0.08tL T = 0.05tL
T = 0.14tL T = 0.10tL
T = 0.20tL T = 0.20tL
0.10 0.10 0.10
NL (!)
NL (!)
NL (!)
0.05 0.05 0.05
T = 0.01tL
T = 0.03tL
T = 0.05tL
T = 0.10tL
T = 0.20tL
0 0 0
1 0.5 0 0.5 1 1.5 1 0.5 0 0.5 1 1.5 2 1.5 1 0.5 0 0.5 1 1.5 2
! ! !
0.3 (d) T = 0.07tH 0.3 0.3 T = 0.07tH
T = 0.20tH (e) T = 0.07tH
T = 0.27tH
(f) T = 0.20tH
T = 0.34tH T = 0.53tH T = 0.34tH
T = 0.67tH T = 0.94tH T = 0.67tH
T = 1.34tH T = 1.34tH T = 1.34tH
0.2 0.2 0.2
NH (!)
NH (!)
01 0 0
0.5 0 0.5 1 1.5 1 0.5 0 0.5 1 1.5 2 1.5 1 0.5 0 0.5 1 1.5 2
! ! !
FIG. 17. Color online: Density of states (DOS) corresponding to the light (a-c) and heavy (d-f) fermion species for a mass imbalance ratio of
= 0.15 for selected U-T cross sections. The temperatures corresponding to the two species are normalized by their respective kinetic energy
scales. At U = 3tL , in the temperature regime under consideration the DOS pertaining to both species shows nonmonotonic thermal evolution.
There is no hard gap at the Fermi level at this interaction since the lowest temperature state correspond to a partially polarized Fermi liquid
(PPFL). At U = 4tL the DOS exhibits non monotonic behavior with increasing temperature and leads to depletion of the spectral weight at
H L
the Fermi level. The onset of non monotonicity marks the temperature scales Tmax and Tmax (see text) corresponding to the heavy and light
species respectively. The inset highlights the nonomonotonic behavior close to the Fermi level. At U = 5tL the thermal evolution of the DOS
L H
is monotonic upto a very high temperature, beyond which the scales Tmax and Tmax (not shown in the figure) sets in
FIG. 18. Color online: Spectral function maps along the {0, 0} to {, } scan across the Brilllouin zone for the (left) light and (heavy) heavy
fermion species at = 0.15 and population imbalance of h=0.6tL , for different U - T cross sections. Notice that at U = 3tL increase in
temperature opens up a gap at the shifted Fermi level in the dispersion spectra corresponding to both species. The heavy species undergoes
faster thermal disordering since it experiences higher scaled temperature.
0.6 150 Within the framework of a lattice fermion model (3D Hubbard
(a) (b) model), it has been found that the first two-body bound state
PPFL PG II is formed at a critical interaction strength of Uc /t 7.9. In-
PPFL TLmax terestingly, quantum Monte carlo (QMC) studies have found
0.4 PG II 100 THmax that for a 3D system the maximum Tc is at U/t 8 [96].
THmax
This brings out the concept that the critical interaction for the
T(tL )
T(nK)
TLmax formation of two body bound state in a lattice fermion model
coincides with the interaction at maximum T c .
0.2 50 PG I In case of 2D gas at continuum a2D as g 0, since
PG I the two-body bound state is formed at any arbitrary inter-
Tc Superfluid Tc Superfluid action. This definition however corresponds to deep inside
the BCS regime where a weak coupling description is valid.
0 0 With increasing interaction the system crosses over to Bose
3 4 5 6 7 8 3 4 5 6 7 8 limit as a2D 0. The coupling at crossover is defined via
U(tL) U(tL) ln(kF a2D ) 0. Interpolation between the BCS and BEC lim-
its showed that maximum T c occurs at ln(kF a2D ) 0, with
T cmax /E F 0.1 [97]. While a 3D like definition (a2D
FIG. 19. Color online: (a) Interaction-temperature (U-T) phase dia- as g 0) puts the unitarity limit in 2D deep inside the BCS
gram at = 0.15 corresponding to the 6Li -40K mixture. The figure
regime, an alternate definition as [ln(kF a2D )]1 is a bet-
shows the Tc scale along with the pseudogap scales for this mixture
at a population imbalance of h = 0.6tL . While the pseudogap fea-
ter choice, firstly because it captures the crossover between
ture in both the fermion species undergoes monotonic thermal evo- the BCS and BEC regimes correctly and also because it cor-
L
lution upto the scale Tmax H
, the monotonicity survives upto Tmax in the responds to the maximum Tc . In other words, the definition
heavier species even though the lighter species is non monotonic in [ln(kF a2D )]1 is adequate to capture the two important
this regime. These two regimes are marked as PG-I and PG-II, re- features of unitarity in 2D, viz. (i) at unitarity neither a pure
spectively. Both the species exhibit pseudogap behavior in the PG-I bosonic nor a fermionic description is sufficient and (ii) the Tc
regime, while in the PG-II regime only the light species is pseudo- is maximum.
gapped. The thermal scales of the individual species are defined w. QMC calculation on 2D Hubbard model have shown that
r. t. their corresponding kinetic energy scales. (b) Thermal scales the maximum Tc is obtained at U/t 5. In our numerical
in terms of the experimental units as would be observable in 6Li -40K simulations we call U/t 4 being close to unitarity where
mixture, in species resolved rf spectroscopy. Close to unitarity (U =
Tc 0.9Tmaxc [77].
4tL ), the pseudogap phase is expected to be observable in both the
species upto T 58nK, beyond which the pseudogap feature sur-
vives only in the light species upto T 108nK. Thus, even though
the Tc 15nk is strongly suppressed in this mixture, short range pair 2. Continuum limit out of lattice model
correlations should be observable upto significantly higher tempera-
tures, in experiments. The present calculations is carried out at a fixed total chem-
ical potential of = 0.2tL where the Fermi surface is dis-
tinctly non circular and the lattice effects are dominant. We
A. Connection to continuum unitary gas observe that even in the limit of low density where the Fermi
surface is circular and k k2 it is difficult to capture the con-
The results presented in this paper are based on a lattice tinuum effects through the lattice model. At interactions close
fermion model while at the same time they are motivated by to unitarity (U 5tL ) even if the Fermi levels occupy the lower
experiments on unitary Fermi gas. In this regard there are few edge of the band, scattering effects couple the states at upper
issues that needs highlighting. We discuss them below. edge. With these high energy states being lattice specific, even
at low enough densities the results obtained do not match with
that of continuum [98, 99]. In order to obtain continuum uni-
1. Concept of unitarity versal physics out of lattice simulations one needs to go to
extremely low densities 0.001, corresponding to lattice size
For the cold atomic gases the interaction strength is quan- of 104 . This is however outside the range of what can be
tified in terms of the s-wave scattering length aD , with D be- attained in the present day.
ing the spatial dimensionality. The corresponding coupling
constant is defined as kF aD , where kF is the Fermi wave vec-
tor. For a 3D gas, the limit of unitarity can be defined as the B. Single channel decomposition
coupling strength at which the first two-body bound state is
formed. With a3D as g gc , where g is the interaction In the present work a single-field decomposition in the pair-
strength, it can be easily seen that 1/kF a3D = 0 at gc , corre- ing channel has been used. In general such a decomposition
sponding to unitarity. At the same time gc corresponds to the can not capture the instabilities in all the channels and one
point across the BCS-BEC crossover where the transition tem- needs to take into account the decomposition in the pairing,
perature is maximum, with T cmax /E F 0.15 for 3D Fermi gas. density and spin channels, particularly in the FFLO regime.
However, in one of our recent works [51] we have shown that
even in the FFLO phase the density channel modulations are
very weak. Moreover, being away from half filling the den-
sity modulations are not as important in the present study as
it would have been at n=1. Decomposition in the additional
magnetic channel might lead to quantitative difference in our
results. However, while such multi-channel decomposition
can be readily incorporated within a mean field formalism,
a non gaussian fluctuation theory like the one presented in
this work would be a difficult feat to achieve with a multi-
channel decomposition. In order to keep the problem numeri-
cally tractable we have chosen for a single channel decompo-
sition. We believe that inclusion of other channels would not
lead to qualitative changes in our results.
1
G LL (k, in ) =
in ((k) + L ) LL (k, in )
1
G HH (k, in ) =
in ((k) + H ) HH (k, in )
where,
| 0 |2 1 FIG. 22. Color online:Dispersion spectrum of the two species in the
LL (k, in ) = [ + LO regime (h=tL ) obtained through the BdG calculation (top panels)
4 ( + (k Q) H ) in comparison to those obtained through Greens function formalism
1 (bottom panels) at different mass imbalance ratio .
]
( + (k + Q) H )
| 0 |2 1
HH (k, in ) = [ +
4 ( + (k Q) L ) Fermi-Fermi mixture comprises of two pseudogap regimes as
1 PG-I, in which the single particle excitation spectra of both
] the species are pseudogapped and PG-II, where only the light
( + (k + Q) L )
species is pseudogapped. We have further investigated the in-
with,ii (k) = 2tii (cos(k x + cos(ky ))) where, ii = L, H. From terplay of population imbalance in such Fermi-Fermi mixtures
the above expressions one can extract the spectral function as, and have shown that at a fixed imbalance in population ho-
ALL (k, ) = (1/)ImG LL (k, + i) |0 . Similar expression mogeneous superfluidity is realized only beyond a critical Uc
can be obtained for AHH (k, ). unlike the balanced superfluid. Moreover, it was shown that a
In Fig.21 and Fig.22 we have compared our results obtained modulated LO superfluid state gives rise to a nodal superfluid
through Monte carlo simulations with those obtained through gap in spite of an s-wave pairing field symmetry. We have
the Greens function formalism at h=0.6tL and h=1.0tL , rep- made quantitative predictions of the thermal scales pertaining
resentative of the BP and LO states, respectively. We have to the 6Li -40K mixture and have suggested that experimen-
shown the spectral function (A (k, )) maps at different mass tal techniques such as rf and momentum resolved photoemis-
imbalance for the light and heavy fermion species. The sion spectroscopy can be used to probe the PG-I regime upto
agreement between the results obtained through the two tech- T58nK and PG-II regime upto T>108nK, in this mixture,
niques is fairly good and along with capturing the species de- close to the unitarity. While the Tc is strongly suppressed in
pendent behavior of the dispersion spectra the technique also this mixture, signatures of short range pair correlation survive
reproduces the multi branched dispersion spectra for the LO upto significantly higher temperatures. We believe that our
state. The agreement justifies our choice of the Greens func- results can serve as suitable benchmarks for the experimental
tion formalism to access quasiparticle behavior at large system observations of 6Li -40K mixture.
sizes, at the ground state.
VI. ACKNOWLEDGEMENT
V. CONCLUSIONS
The author gratefully acknowledges Prof. Pinaki Majum-
In conclusion, we have investigated the BCS-BEC dar for his insightful comments on the manuscript. The HPC
crossover of mass imbalanced Fermi-Fermi mixture within the cluster facility of HRI, Allahabad is duly acknowledged. A
framework of a two-dimensional lattice fermion model. We part of this work was carried out at IMSc, Chennai, India and
have mapped out the thermal phase diagram in the -T plane the author acknowledges the hospitality provided during the
and have shown how the thermal scales are suppressed by the visit.
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