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Chemical Engineering and Processing 45 (2006) 461470
Received 27 July 2004; received in revised form 3 November 2005; accepted 3 November 2005
Available online 28 December 2005
Abstract
Spray drying operations with rotary disc atomizers as well as pressure nozzles as atomizing devices are widely used in diverse industries. The
design of spray dryers is typically optimized for the design conditions. However, users sometimes need to use the same spray dryer chamber with
some modifications due to the requirements of different products and or production rates. In this paper, we present results of a computational fluid
dynamic study carried out to investigate the possibility of multi-functional applications of a specific spray dryer chamber. The predicted airflow
pattern is validated by favorable comparison with published data. The airflow pattern and temperature distributions predicted by the model at
different levels in the drying chamber are presented and discussed. The effects of different atomizer designs are also investigated. Note that the
two types of atomizers yield very different droplet size distributions as well as spray patterns. The volumetric evaporation rate values, heat transfer
intensity and thermal energy consumption per unit evaporation are computed and compared for drying of a 42.5% solids maltodextrin suspension
in a spray chamber 2.2 m in diameter with a cylindrical top section 2.0 m high and a bottom cone 1.7 m high. Wall regions most susceptible to
formation of undesirable deposits are also identified. Computed droplet trajectories for the two spray patterns are shown to display very different
flow, temperature and drying characteristics.
2005 Elsevier B.V. All rights reserved.
Keywords: Atomization; Drying; Flow pattern; Heat and mass transfer; Turbulence model
0255-2701/$ see front matter 2005 Elsevier B.V. All rights reserved.
doi:10.1016/j.cep.2005.11.004
462 L.X. Huang et al. / Chemical Engineering and Processing 45 (2006) 461470
spray dryer. Kieviet et al. [12,13] investigated a co-current spray equation and the species conservation equation. Two-way cou-
dryer fitted with a pressure nozzle both in CFD simulation and pling between drying medium and droplet is considered as well.
experiments. The CFX code was used. More recently, Huang et The general equation for an axial symmetrical flow in cylin-
al. [14] investigated the effects of different chamber geometries, drical coordinates can be written as:
i.e., cylinder-on-cone, lantern, hour-glass and pure cone, on the
(U) 1 (rV)
drying performance and particle residence time using FLUENT +
code. They showed that it was possible for the designer to select x r r
other chamber geometries, and not only the traditional cylinder- 1
= + r + S + Sp (1)
on-cone geometry. Huang et al. [15] also carried out a parametric x r r r r
study for a co-current spray dryer fitted with pressure nozzle. A
ultrasonic nozzle spray dryer was studied numerically by Huang where S is the source term of gas phase, Sp the source term of
et al. [16], as well. Goula and Adamopoulos [17] also used FLU- the droplet phase and the effective viscosity, , is summarized
ENT to simulate a lab-scale spray dryer. in Table 1.
However, previous workers focused attention on spray dryers The turbulence viscosity T is computed by:
fitted with nozzles, in particular, the pressure nozzle atomizers.
k2
Few studies on spray dryers with rotary disc atomizers can T = C g (2)
be found in the literature; most of them are experimental in
nature. Huang et al. [18] showed that the RNG k different The generation of turbulence, Mk , is given as follows:
turbulence model is suitable for simulating the complex,
2
swirling two-phase flow in the spray drying chamber fitted U V 2 U 2 V 2 V
with a rotating disc when compared with three other turbulence Mk = T + +2 + +
r x x r r
models, i.e., standard k, realizable k and Reynolds stress
models using FLUENT code [19]. W 2 W W 2
The objective of this work is to present and discuss a set of + + (3)
x r r
numerical results obtained using the CFD code Fluent 6.1 for a
co-current flow spray dryer fitted with either a rotary disk or a
pressure nozzle [19]. A fully three-dimensional configuration, The empirical constants of the turbulence model are taken
i.e., cylinder-on-cone geometry, is considered. The RNG k from the standard constants given by Launder and Spalding [20].
different turbulence model was selected in this study based on The combined EulerLagrangian approach is used to obtain
our previous work [18]. Comparison with limited experimental the particle trajectories by solving the force balance equation for
data is included as well. the particles considering the discrete phase inertia, aerodynamic
drag, gravity gi and other optional user-defined forces Fxi .
2. The mathematical model dupi 18 Re g
= CD (ui upi ) + gi + Fxi (4)
dt p dp 24 g
The hybrid Eulerian and Lagrangian approach is used to
model the heat and mass transfer between two-phase flow (air and the relative Reynolds number
and droplet) in spray drying process. This computation involves
numerical solution of the discretized continuity equation, the dp |up u|
Re = (5)
momentum equations with suitable turbulence model, energy
Table 1
Terms in the general equations
Equation S Sp
dmp
Continuity 1 0 0
U 1 V
P
dt
Axial momentum U + T + r + RU
x x r r x x
U
1
V P g W 2 2V
Radial momentum V + T + r + RV 2
x r r r r r r r
2
Tangential momentum W + T (rW) + RW
T r r
Turbulence energy k + Mk g
kT
Dissipation rate of turbulence kinetic energy + (C1 Mk C2 g )
k
T
Enthapy n + Rn
n
T dmp
Vapor mass faction H + RH
H dt
L.X. Huang et al. / Chemical Engineering and Processing 45 (2006) 461470 463
The mass transfer between the gas and the droplet are calcu- Chamber wall thickness (m) 0.002
lated according to the following equation: Wall material Steel
Wall-heat transfer coefficient (W/m2 K) 3.5
Air temperature outside wall ( C) 27
dmp
= kc Ap (Cs C ) (8) Interaction B.C. between wall and droplet Escapea
dt a Indicates that the particles are lost from the calculation domain at the point
The heat and mass transfer coefficient can be obtained from of impact with the wall.
Eqs. (9a) and (9b) with suitable coefficient values for , , , ,
and . These values are obtained from several sources [21,22].
The FLUENT code solves the governing equations listed 3. Boundary conditions and atomization models
here.
3.1. Boundary conditions
Nu = 2 + Re Pr (9a)
The simulations were performed for steady state operation.
Sh = 2 + Re Sc (9b) The grid-independence of the results was demonstrated using
different mesh sizes, i.e., 0.03, 0.015 and 0.0075 mm. Finally,
The second period, called droplet boiling, is applied to predict 0.015 mm mesh size is selected in this paper. The chamber is
the convective boiling of a discrete phase droplet when the tem- a cylinder-on-cone vessel, 2.215 m in diameter with a cylindri-
perature of the droplet has reached the boiling point and while cal top section, 2.0 m high and a bottom cone, 1.725 m high.
the mass of the droplet exceeds the non-volatile fraction. The The angle of the bottom cone is 60 . The atomizer is installed
boiling rate equation is applied [FLUENT [19]]: at the top of the drying chamber. Air is blown into it from the
top center as shown in Fig. 1. The feed is a 42.5% solids mal-
d(dp ) 4k Cp, (T Tp )
= (1 + 0.23 Red ) ln 1 + todextrin suspension. The boundary conditions at the inlet, the
dt p cp, dp hfg outlet, chamber wall and the turbulence model are summarized
(10) in Table 2.
G0.24
d = 1.4 104 L
0.83
(11)
(NdD ) (ndh )0.12
Fig. 3. Comparison of temperature profiles between prediction and Kieveits Fig. 4. Comparison of humidity profiles between prediction and Kieviets mea-
measurement [13] at spray condition. surement [13] at spray condition.
From the humidity profiles at the 0.3 and 1.4 m levels shown
in Fig. 4, it is also seen that a large variation of humidity occurs
in the central column. This also indicates that rapid drying takes
place in this region. The remaining volume has almost constant
humidity. This result implies that these regions are not effectively
used for drying and so there are opportunities here to improve
the design and operation.
It is also observed that the humidity profiles at 0.3 m level Fig. 5. Comparison of velocity profiles for a spray dryer fitted with pressure
and 1.4 m level along X-axis are symmetric and are asymmet- nozzle and rotary disk.
466 L.X. Huang et al. / Chemical Engineering and Processing 45 (2006) 461470
ric at 1.4 m level along Y-axis. It implies that the evaporation In Fig. 5, it is noted that the velocity profiles are nearly sym-
occurs non-uniformly at the cross-section of the drying cham- metric at 0.3 and 1.4 m levels for Case A. On the other hand,
ber. It also shows that the symmetric model may not give too asymmetric velocity profiles are found in Case B. It is also found
accurate predicted results. that the absolute velocity is higher in Case B at 0.3 m level than
in Case A. It is due to the disc rotating which induce the air high
4.5. Comparison of a spray dryer tted with a pressure swirl. However, when the air passes downward, such as at 1.4 m
nozzle and a rotating disk level, the high velocity zone only slightly expands in Case A.
Case B at 1.4 m level presents a larger high velocity zone than
4.5.1. Comparison of velocity proles and air ow patterns that in Case A.
between a spray dryer tted with a pressure nozzle (Case A) If the axial velocity profiles in Fig. 6 are considered, it is
and rotating disk atomizer (Case B) observed that there is a reverse flow at 0.3 m level in Case B
The velocity magnitude and axial velocity profiles for a spray which is not present in Case A. It is due to the rotating disk which
dryer (SD) fitted with a pressure nozzle (PN) and a rotating pulls the air below the disk upwards. This phenomenon was
disk (DK) are shown in Figs. 5 and 6, respectively. We named also observed by Masters [23] and was named as air pumping
the a spray dryer fitted with PN as Case A and DK as Case B. effects. These reverse flows disappeared rapidly as the drying air
Generally, it is found that the high variation of velocity is located proceeds downwards, e.g., at 0.6 m level (Fig. 6b). However, at
at the center core of diameter of 0.3 m as what we found in no the same time, there is a reverse flow formed near the chamber
spray condition [Fig. 2]. wall as shown in Fig. 6b and c. At the 1.4 m level, these side
Fig. 6. Comparison of axial velocity profiles for a spray dryer fitted with pressure Fig. 7. Comparison of temperature profiles for a spray dryer fitted with pressure
nozzle and rotary disk. nozzle and rotary disk.
L.X. Huang et al. / Chemical Engineering and Processing 45 (2006) 461470 467
reverse flows are more obvious and strong in Cases A and B. higher volumetric effectiveness of the chamber [14]. We also
This shows that air recirculation appears at this level. The radial find that the temperature variation is quite large in the top region
and tangential velocity profiles (not shown here) show that the of the chamber in Case B.
flows are too complex to identify typical flow patterns.
4.5.3. Comparison of humidity proles for Cases A
4.5.2. Comparison of temperature proles for Cases A and B
and B Fig. 9 displays humidity profiles for Cases A and B at different
The temperature profiles for Cases A and B are shown in levels in the drying chamber. From Fig. 9a, it is noted that the
Fig. 7. It is seen that the temperatures in the central core of humidity in the central core of diameter 0.2 at 0.3 m level in
diameter of 0.2 m are almost the same at 0.3 m level in both Case B is lower than that in Case A. However, this humidity is
cases, but radial variations are larger in Case B than those in Case larger in Case B as the radius increases than that in Case A. This
A. It is because the rotating disk provides a horizontal spray. At is mainly due to the radially directed spray for rotating disk and
0.6 m level (Fig. 7b), it shows almost the same conclusions as downward spray for pressure nozzle. Thus intense evaporation
those for the 0.3 m level. At 1.4 m level (Fig. 7c), Case A gives occurs at different locations because of the designs of different
a lower temperature profile in the central core than Case B. It is atomizers. At 0.6 m level (Fig. 9b), the same conclusion can be
due to the evaporation which takes place in this region since the made.
pressure nozzle provides a downward spray. However, Case B However, Case A presents a more uniform humidity profiles
presents a slightly wider region of high temperature than Case at 1.4 m level than in Case B. It is due to the stronger recirculation
A. It is probably because the rotating disk produces a stronger in Case A, which makes the high humidity air at the lower section
swirling flow and makes the high temperature zone to expand. travel upwards. On the other hand, Case B presents lower humid-
Fig. 8 shows the temperature contours in planes YZ and XZ ity in the central core and high humidity outside this core. Such
for Cases A and B. They indicate that the temperature variation is a condition may lead to less evaporation because the droplets
limited within the narrow central region for Case A and occupies always pass through a high humidity and lower temperature dif-
more regions for Case B. This implies that Case B may yield ference zone.
Fig. 8. Comparison of temperature contours for a spray dryer fitted with pressure nozzle and rotary disk.
468 L.X. Huang et al. / Chemical Engineering and Processing 45 (2006) 461470
Table 3
The overall drying performance for nozzle and disc spray dryers
Cases Case A Case B Case C
it directly leads to lower evaporation rate for a rotating disk Appendix A. Nomenclature
SD. The droplet size distribution is obtained from a pressure
nozzle. However, the rotating disk atomizer normally gives a a1 , a2 and a3 constants
smaller mean droplet size and a narrower size distribution than Ap surface area of the droplet (m2 )
a pressure nozzle [23]. The evaporation rate may be increased CD drag coefficient
in Case B if the fine mean droplet and narrow size distribution Cs moisture concentration at the droplet surface (mol/m3 )
which is produced by a rotating disk are used. Case C is designed Cg moisture concentration in the bulk gas (mol/m3 )
for this purpose. Case C is different from Case B only in terms Dm diffusion coefficient of vapor in the bulk (m2 /s)
of the droplet size distribution and mean droplet size, i.e., the cp heat capacity of the droplet (J/kg K)
minimum droplet diameter of 10 m and the maximum droplet dp droplet diameter (m)
diameter of 100 m with an average droplet diameter Dm of d Sauter mean droplet diameter (m)
50 m are used in Case C [23]. dh holes diameter or vane height in disk (m)
The predicted results shown in Table 3 confirm the above dD rotating disk diameter (m)
conclusion, i.e., a higher evaporation rate is obtained in Case dmp
dt rate of evaporation (kg/s)
C due to the small mean droplet size and narrow droplet size
Fxi user-defined-function in particle tracking governing
distribution. The evaporation rate is increased about 4% higher in
equation
Case C than that in Case B. Considering the deposit percentage in
gi gravity component (m2 /s)
Cases B and C, we find that only the deposits on the cylinder wall
Gk production of turbulence kinetic energy due to the mean
are increased significantly. It is probably because the smaller
velocity gradients
particles are easily carried by the drying medium since there is
G production of turbulence kinetic energy due to buoy-
a strong swirling flow in the upper volume of the chamber.
ancy
Because of the higher evaporation rate in Case C, a lower
GL mass feed flow rate (kg/h)
residual moisture in product is obtained as well compared with
h convective heat transfer coefficient (W/m2 K)
those in Cases A and B. The energy consumption values per
hfg latent heat (J/kg)
unit evaporation are almost the same in Cases A, B and C. It
k turbulent kinetic energy (m2 /s2 )
indicates that the narrower droplet size distribution and smaller
kc mass transfer coefficient (m/s)
mean droplet size in spray drying better the overall drying per-
keff effective thermal conductivity of gas (W/m K)
formance.
kg thermal conductivity of the hot medium (W/m K)
mp mass of the droplet (kg)
5. Conclusions
n number of holes or vanes in disk
N disk rotating speed (rpm)
A three-dimensional computational fluid dynamic model for
Ni molar flux of vapor (mol/m2 s)
pressure nozzle and rotating disc spray dryers was developed and
RU , RV and RW user-defined source term in momentum equation
investigated. Good agreement with limited experimental data is
Rn user-defined source term in energy equation
obtained considering complexity of the system studied. It also
Sk user-defined source term
shows that a three-dimensional model is more suitable for such
S user-defined source term
a spray drying system than a two-dimensional axi-symmetric
t time (s)
model [12,13,15].
T temperature (K)
The results obtained from the 3D CFD model are presented in
Tg gas temperature (K)
terms of the velocity magnitudes, velocity components, temper-
ui gas velocity vector (m/s)
ature profiles, humidity profiles and particle trajectories. Results
up droplet velocity vector (m/s)
show that the flow patterns in a SD are very complex. Pressure
nozzle may lead to a high velocity variation core formed in the
center of the chamber. Large recirculation is also found in a Greek letters
pressure nozzle SD. surface tension (N/m)
It is also observed that a greater proportion of the chamber gas density (kg/m3 )
volume is utilized in a rotary disc atomizer SD than in one fit- p droplet density (kg/m3 )
ted with a pressure nozzle SD. There are some regions that are viscosity (kg/m s)
deposit-free in the chamber near cylinder wall in a pressure noz- energy dissipation rate (m2 /s3 )
zle SD. Larger zones of deposits on cylinder wall are found for k turbulent Prandtl number for k
a rotating disk SD and on internal bend and a conical wall for a turbulent Prandtl number for
pressure nozzle SD. These predicted results show that a larger- t turbulent viscosity
diameter chamber should be used for a SD fitted with DK and a
tall small-diameter one for one fitted with PN. Subscripts
From predicted results, it is found that the narrower droplet g air
size distribution and smaller mean droplet diameter present bet- p droplet
ter overall drying performance. C constant
470 L.X. Huang et al. / Chemical Engineering and Processing 45 (2006) 461470
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