A.

MAX DOAS
DOAS
DOAS
[1-7] DOAS
DOAS DOAS DOAS
DOAS

DOAS

MAX DOAS

[8-13] MAX DOAS

[9-27]
U.Platt MAX DOAS

[8]
,X. Li[11]
MAX DOAS H. IrieR.
Sinreich[16,17]T. WagnerU. Frie
[18,19] P. WangR. J. LeighH. Leser R.

Sinreich [20-23]
[5,24,25]

[26,27]

B.

1 M 0

 M 1 M 1

N p g Pm
[14,15]
Pa
Pa R M 1 M 0
R F p g , N , , Pa , Pm , ,

(1)

p g N

Pa

Pm

p g Pa Pm h Pg

Pg = p g N R

[4-7]

S p g N Pa Pm

S F p g , N , , Pa , Pm , ,

(2)

N Pm h

Pa

 (2) p g

p g p g

p g
p g

p g

[1]. Chan MH, Andrew YSC, Measurement of atmospheric nitrogen dioxide column density by
solar spectroscopy method . SPIE, 2005, 5832: 283
[2]. G. Honninger, H. Leser, et al, Groundbased measurements of halogen oxides at the Hudson
Bay by active long path DOAS and passive MAX-DOAS. GEOPHYS RES LETT, 2004, 31:
L04111
[3]. F. Lohberger, G. Honninger, et al, Ground based Imaging Differential Optical Absorption
Spectroscopy of atmospheric gases . APPL OPTICS, 2004, 43: 4711
[4]. NO2 2000,
492507
[5].
2006261356
[6].
2006, 551530
[7]. DOAS
2008282417

[8]. G. Honninger, C. von Friedeburg, et al, Multi axis differential optical absorption
spectroscopy (MAX-DOAS). ATMOS CHEM PHYS, 2004, 4: 231
[9]. NO2
2010302464
[10]. MAX-DOAS 20094
387
[11]. X. Li, T. Brauers, et al, MAX-DOAS measurements in southern China: 1. automated
aerosol profile retrieval using oxygen dimers absorptions. ATMOS CHEM PHYS, 2008, 8: 17661
[12]. F. Wittrock, H. Oetjen, et al, MAX-DOAS measurements of atmospheric trace gases in NyAlesund - Radiative transfer studies and their application. ATMOS CHEM PHYS, 2004, 4: 955
[13]. A. Heckel, A. Richter, et al, MAX-DOAS measurements of formaldehyde in the Po-Valley.
ATMOS CHEM PHYS, 2005, 5: 909
[14]. C. Von Friedeburg, Derivation of Trace Gas Information combining Differential Optical
Absorption Spectroscopy with Radiative Transfer Modelling. PhD-thesis , 2003
[15]. G. Honninger, Halogen Oxide Studies in the Boundary Layer by Multi Axis Differential
Optical Absorption Spectroscopy and Active Longpath-DOAS. PhD-thesis , 2002
[16]. H. Irie, Y. Kanaya, et al, First retrieval of tropospheric aerosol profiles using MAX-DOAS
and comparison with lidar and

sky radiometer measurements. ATMOS CHEM PHYS, 2008, 8:

341
[17]. R. Sinreich, U. Frie, et al, Retrieval of Aerosol Distributions by Multi-Axis Differential
Absorption Spectroscopy (MAX-DOAS). SPRINGER, 2007, 1145
[18]. T. Wagner, B. Dix, et al, MAX-DOAS O 4 measurements: A new technique to derive
information on atmospheric aerosols-Principles and information content. J GEOPHYS RES,
2004, 109: D22205
[19]. U. Frie, P. S. Monks, et al, MAX-DOAS O4 measurements: A new technique to derive
information on atmospheric aerosols: 2. Modeling studies. J GEOPHYS RES, 2006, 11: D14203
[20]. P. Wang, A. Richter et al, Measurements of tropospheric NO2 with an airborne multi-axis
DOAS instrument. ATMOS CHEM PHYS, 2005, 5: 337
[21]. R. J. Leigh, G. K. Corlett, et al, Concurrent multi-axis differential optical absorption
spectroscopy system for the measurement of tropospheric nitrogen dioxide. APPL OPTICS,

2006, 45: 7504

[22]. H. Leser, G. Honninger, et al, MAX-DOAS measurements of BrO and NO 2 in the marine
boundary layer. GEOPHYS RES LETT, 2003, 30: 1537
[23]. R. Sinreich, U. Frie, et al, Multi axis differential optical absorption spectroscopy (MAXDOAS) of gas and aerosol distributions. FARADAY DISCUSS, 2005, 130, doi:10.1039/b419274
[24]. Zuo HY, Liu QJ, et al, Equiangular method: a technique of multiaxis DOAS. J OPT
SOC AM B, 2009, 26: 1656
[25]. Zuo HY, Zhu SF, et al, Retrieval of the vertical column density of the atmospheric
pollution gases by using the scattered solar radiation. J QUANT SPECTROSC RA, 2008, 109:
2628
[26]. E. Palazzi, Retrieval of trace gases vertical profile in the lower atmosphere combining
Differential Optical Absorption Spectroscopy with radiative transfer models. PhD-thesis , 2008
[27]. N. Theys, M. Van Roozendael, et al, Retrieval of stratospheric and tropospheric BrO
columns from multi-axis DOAS measure- ments at Reunion Island (21 S, 56 E). ATMOS
CHEM PHYS, 2007, 7: 4733
[28]. Zuo HY, Luo SR, et al, A technique to improve the accuracy of retrieval of the aerosol
size- distribution. OPT LETT, 2010, 35: 1380
[29]. Zuo HY, Luo SR, et al, Retrieve the aerosol size-distribution by using a combined
model. OPT LASER TECHNOL, 2010, 42: 535
[30]. 1995
[31].
2007, 56 6132
[32]. 2004, 31
224

[26]

1,


p g

50KM
50KM50KM [14]
50KM

a. p g h h
p g h

b. [ 1]

h Ei
p g h h Bi exp
Ti
i 1

(3)

M
M 3
[28,29] p g h

Bi Ei Ti

p g h
[28,29]

[30]

a.
NO2 20

 20 pi i 1,2,3 20
20
50KM 5 1
5 20
3

3 NO2

1 20

DOAS NO2 N
NO2
2 Pa

Pm

3 Pm Mie
C m n n n

 Dm n,

4 Pa Mie
C a n
Da n, [ 2]

4 n

4 20 N
NO2 NO2 A n
5
C m n C a n Dm n, Da n, A n

20

20
4 20
45

 2 C m n C a n

4 n
C m n sin
C a n sin

Dm n, 2 Da n, 2

A n sin

b.
n
4
1 A n

sin

NO2 [

3] 2,3
2
2 C m n sin
3

Dm n, 2

0< <180 n -1
180< <360 n +1
3
3 C a n sin

Da n, 2

0< <180 n -1
180< <360 n +1

n +1 1- A n

sin

- C g n sin - C a n sin

n -1 n +1
2 3
0180 360

[8] M 1 M 0 DOAS
NO2