Professional Documents
Culture Documents
July 2014
Certificate
This is to certify that, Prakash Mandal, RSE, OCES-2013, BARC Training School, Mumbai has
completed his Project Work under my guidance.
Signature _____________________________
Name & Designation_____________________
Division/Unit_________________________________
Acknowledgements
The work described in this Mini Project thesis has been carried out under the
guidance and supervision of Dr. R. K. Gopalakrishnan, Head RHCS RSSD, BARC
Mumbai, between May 2014 and July 2014.
I express my sincere thanks and gratitude to him for his constant guidance,
motivation, suggestions and discussions throughout this work.
I specially thank Shri Amit Bhatnagar RHCS Dhruva who helped me in
each and every step for doing this project. Apart from the academic guidance, his
friendly nature was a boost to my spirit to move ahead constantly.
I am thankful to Dr. K. S. Pradeepkumar Head RSSD for his suggestion and
motivation.
I specially thank my friends and lab mates for helping me. It has been a
pleasure to work in company of good people of the unit. My sincere thanks and
regards to Mr. N. Kalyansundarm RSO Dhruva for his kind help at various stages
in my project. I thank all my batchmates and friends for their constant support
which has given me the confidence for moving ahead across any difficulties. I
finally thank all my teachers and professors of training school, who have made me
capable to do whatever I am able to do today. Lastly, I would like to express my
gratitude to my parents, grandparents and my sister. All that I have accomplished
in my life is the result of their care and support.
PrakashManldal
BARC Mumbai
July, 2014
Table of Contents
Page Number
1. Abstract
1. Introduction
4. Exposure pathways
10
11
13
14
16
17
18
19
20
21
21
22
12.
23
11. Conclusion
25
12. References
25
1.1 Abstract: Research reactors are required for neutron research applications,
isotope production, reactor material testing, etc. During normal reactor operation
dose to the member of public and workers are insignificant. But in a rare event of a
reactor accident condition, the dose to the occupational workers and members of
the public can be large. It is required to estimate the dose to members of the public
in the event of an accident scenario. In this work, dose rate at different distances
has been estimated in hypothetical condition of accident in design and beyond
design basis accident. This project aims to calculate the dose from Fission Product
Noble Gases (FPNG) and iodine at various distance from nuclear facility in various
modes of exposure scenario. Dose in DBA and BDBA condition has been
compared. It is expected that this study would help in emergency preparedness
and planning.
1.2 Introduction
Radiological impact due to atmospheric releases following a hypothetical nuclear
accident for a 100 MW research reactor is analyzed with following assumptions.
1.
2.
3.
4.
5.
Assumptions:
For the calculation of dose in accidental condition, a hypothetical scenario is taken
into account. The following assumptions are made ( a) 43% of total fuel inventory
will lose its integrity and will have clad failure (b) From these fuels 100% fission
product noble gas (FPNG), 25% iodine and 1% particulate will get released into
primary coolant (c) ECCS is available (d) All FPNG will get released into the
containment (e) Partition factor of 700 is used for iodine release to containment.
As the emergency exhaust system is initiated, activity of containment will be
released to atmosphere through 100 m stack. All ventilation will be through
Charcoal and HEPA filter. Efficiency of charcoal filter is taken as 90% and HEPA
as 99% while calculating released activity.
Pressurisation is not envisaged due to the credit of Emergency exhaust system. A
leak rate of 0.2% V/V-hr has been taken into calculation for duration of 12 min.
Calculation has been done for weather category F with a wind speed 2 m/sec for
ground release and 4.3 m/s for stack release.
For beyond design basis accident, no credit has been given to charcoal filter.
Organ
Whole body
Childs Thyroid
Dose Limit
100 mSv
500 mSv
Power
Coolant
Moderator
Fuel
Clad
n-flux
Coolant inlet temperature
Coolant outlet temperature
No of coolant channels
No of fuel assembly
Reactor building volume
Burn-up (Average)
100MW
D2O
D2O
Nat-U metal
Al
1.8E+14
45C
75C
146
127
55,000m3
1000 MWD/T
1.8 General feature of the reactor: For the estimation of radiological imapact in
a hypothetical accidental scenario, a single containment 100 MW research reactor
was considered.
1.9 Barriers to release of radioactivity: There are several barriers for the release
of radioactivity from fuel matrix to the environment.
1.10 Introduction about the reactor: For the dose estimation, considered reactor
is a 100MW thermal neutron, vertical core, heterogeneous, tank type, U-natural
fuelled, heavy water moderated, cooled and reflected multipurpose research
Dose is estimated up
to 1.6 Km, for stability
class F plume will not
touch the ground up
to that distance so
the dose, contributed
by ground deposition
will be negligible.
Reactor type
Reactor size or power level
Fuel characteristics
Reactor utilization
Nature of Accident
Group
Half life
Core inventory
(Ci)
Kr-83m
Kr-85m
Kr-85
Kr-87
Kr-88
Kr-89
Kr-90
Kr-91
Kr-92
Noble gas
Noble gas
Noble gas
Noble gas
Noble gas
Noble gas
Noble gas
Noble gas
Noble gas
114m
4.4h
10.6y
78m
2.8h
3.2m
33s
10s
3s
4.44E+05
1.06E+06
2.56E+03
2.14E+06
3.01E+06
3.85E+06
3.82E+06
2.87E+06
1.26E+06
Xe-131m
Xe-133m
Xe-133
Xe-135m
Xe-135
Xe-137
Xe-138
Xe-139
Xe-140
Noble gas
Noble gas
Noble gas
Noble gas
Noble gas
Noble gas
Noble gas
Noble gas
Noble gas
12d
2.3d
5.27d
15.3m
9h
3.9m
17m
41s
16s
2.47E+04
1.64E+05
5.61E+06
9.45E+05
2.36E+06
4.99E+06
5.20E+06
4.26E+06
3.00E+06
I-129
I-131
I-132
I-133
I-134
I-135
I-136
I-137
I-138
I-139
Halogen
Halogen
Halogen
Halogen
Halogen
Halogen
Halogen
Halogen
Halogen
Halogen
17000000y
8.05d
2.3h
20.8h
52.5m
6.7h
86s
24.4s
6.3s
2s
4.10E-03
2.36E+06
3.56E+06
5.61E+06
6.33E+06
5.25E+06
2.52E+06
2.71E+06
1.37E+06
6.24E+05
11
Sr-89
Sr-90
Sr-91
Sr-92
Sr-93
Sr-94
Strontium group
Strontium group
Strontium group
Strontium group
Strontium group
Strontium group
50.5d
28y
9.7y
2.7h
7.9m
1.3m
2.36E+06
2.02E+04
4.86E+06
4.97E+06
5.29E+06
4.90E+06
Te-125m
Te-127m
Te-127
Te-129m
Te-129
Te-131m
Te-131
Te-132m
Te-133m
Te-134
Tellurium group
Tellurium group
Tellurium group
Tellurium group
Tellurium group
Tellurium group
Tellurium group
Tellurium group
Tellurium group
Tellurium group
58d
105d
9.3h
37d
72m
30h
24m
77h
52m
43m
7.75E+01
5.18E+03
1.09E+05
5.99E+04
5.28E+05
3.02E+05
2.13E+06
3.54E+06
2.49E+06
5.61E+06
Cs-134
Cs-135
Cs-136
Cs-137
Cs-138
Cs-139
Cs-140
Alkali metal
Alkali metal
Alkali metal
Alkali metal
Alkali metal
Alkali metal
Alkali metal
2.2y
2600000y
12.9d
30y
32.2m
9.5m
66s
3.24E+02
1.25E-06
5.87E+03
2.09E+04
5.61E+06
5.32E+06
4.82E+06
Ru-103
Ru-105
Ru-106
Ru-107
Ru-103m
Noble metal
Noble metal
Noble metal
Noble metal
Noble metal
1.79E+06
8.70E+05
3.97E+04
1.55E+05
1.62E+06
Ce-141
Ce-143
Ce-144
Ce-145
Ce-146
Cerium group
Cerium group
Cerium group
Cerium group
Cerium group
3.66E+06
4.93E+06
6.61E+05
3.25E+06
6.62E+03
Zr-95
Zr-97
Lanthanide
Lanthanide
2.69E+06
4.87E+06
12
13
exp (
)exp (
) exp (
)....(2)
where
, and
are the standard deviations of concentration distribution along
the tree axes and Q is the source strength or the quantity of material released (Bq).
Time integrated concentration (TIC) , at a downwind point along the x-axis
over a period constituting complete passage of the cloud by integrating the above
equation using the transformation x=ut, we get
( , , , )=
exp (
) exp (
) ..(3)
Where,
U=mean wind speed at the height of release (m/s).
1.19 Continuous point source: For a continuous point source of strength Q`
(Bq/s) situated at the origin of a fixed co-ordinate system in which x-axis is in
downwind direction , y-axis is in horizontal crosswind direction and z-axis in the
vertical direction, the concentration at a point (x,y,z) is given by
( , , )=
exp (
) exp (
.(4)
Where
and
are the standard deviations of the concentrations at distance x in
the horizontal crosswind direction and in vertical direction respectively. These are
14
. (5)
Shifting the co-ordinate system from effective stack height level to the base of the
stack the equation (3) is transformed to
( , , ) =
`
2
exp (
){exp (
+exp (
2
( + )
)}...(6)
The additional exponential term takes account of the fact that ground being
impervious to the radioactive material would reflect the plume. The effect of
reflection is taken into account by considering a virtual source at a depth H below
the ground.
Special cases:
(i) Expression for ground level concentration (GLC) is obtained by setting z=0 in
equation (5), we get
( , , 0) =
exp (
)exp (
......(7)
(ii) expression for plume centerline concentration is obtained by setting y=0 in the
above equation yielding :
( , 0,0) =
exp (
.(8)
15
1.21 Wind speed correction with height: wind speed and direction change with
height. Wind speed to be used in the diffusion expression is the one at the effective
height of release H. Standard height for national networks recommended by World
Meteorological Organization is 10 metres above ground.
The power law of wind profile is expressed as:
Where
( )
( )=(
) ..(9)
: n=0.5
16
1.23 The effective dose rate from immersion in a radioactive cloud is given by:
Dim = CA DFim
...(10)
where
2.0 CALCULATION:
2.1 Evaluation of effective stack height for different stability class: Formula
used
=
+ ( )
( +
.(11)
(2 )
Table 5: Effective stack height and wind speed for different stability class
Stack
height
(m)
100
100
100
Stability n-value
class
unstable
neutral
stable
0.2
0.25
0.5
p-value
0.11
0.14
0.33
17
wind speed
at 100m
(m/s)
(m)
2.58
2.77
4.30
104.4
104.2
103.2
Core
inventory
43% fail
100%
1%
25%
FPNG (water)
Iodine
(water)
100%
Containment
Particulates
(water)
0.143%
Containment
0.001%
Containment
Fig 7: Percentage of activity transfer considered for the hypothetical nuclear accident
core
equilibrium
activity (Ci)
activity in
coolant (Ci)
activity in
water (Ci)
I-129
4.10E-03
1.76E-03
4.40E-04
I-131
2.36E+06
1.01E+06
2.54E+05
I-132
3.56E+06
1.53E+06
3.82E+05
I-133
5.61E+06
2.41E+06
6.03E+05
I-134
6.33E+06
2.72E+06
6.81E+05
I-135
5.25E+06
2.26E+06
5.64E+05
I-136
2.52E+06
1.08E+06
2.71E+05
I-137
2.71E+06
1.17E+06
2.91E+05
I-138
1.37E+06
5.89E+05
1.47E+05
I-139
6.24E+05
2.68E+05
6.71E+04
FPNG 43% from fuel to coolant then 100% up to stack
18
activity in
containment
(Ci)
Stack
Stack
release(Ci) release in
Bq
6.30E-07
3.63E+02
5.46E+02
8.63E+02
9.73E+02
8.07E+02
3.88E+02
4.17E+02
2.11E+02
9.59E+01
3.15E-10
1.81E-01
2.73E-01
4.31E-01
4.87E-01
4.03E-01
1.94E-01
2.08E-01
1.05E-01
4.80E-02
1.16E+01
6.71E+09
1.01E+10
1.60E+10
1.80E+10
1.49E+10
7.17E+09
7.71E+09
3.90E+09
1.77E+09
release
Kr-83m
4.44E+05
1.91E+05
1.91E+05
Kr-85m
1.06E+06
4.54E+05
4.54E+05
Kr-85
2.56E+03
1.10E+03
1.10E+03
Kr-87
2.14E+06
9.20E+05
9.20E+05
Kr-88
3.01E+06
1.30E+06
1.30E+06
Kr-89
3.85E+06
1.65E+06
1.65E+06
Kr-90
3.82E+06
1.64E+06
1.64E+06
Kr-91
2.87E+06
1.23E+06
1.23E+06
Kr-92
1.26E+06
5.41E+05
5.41E+05
Xe-131m
2.47E+04
1.06E+04
1.06E+04
Xe-133m
1.64E+05
7.03E+04
7.03E+04
Xe-133
5.61E+06
2.41E+06
2.41E+06
Xe-135m
9.45E+05
4.06E+05
4.06E+05
Xe-135
2.36E+06
1.01E+06
1.01E+06
Xe-137
4.99E+06
2.14E+06
2.14E+06
Xe-138
5.20E+06
2.24E+06
2.24E+06
Xe-139
4.26E+06
1.83E+06
1.83E+06
Xe-140
3.00E+06
1.29E+06
1.29E+06
Particulates, 43%to coolant, 1%to water, 0.001%to
containment
Cs-134
3.24E+02
1.39E+02
1.39E+00
Cs-135
1.25E-06
5.38E-07
5.38E-09
Cs-136
5.87E+03
2.52E+03
2.52E+01
Cs-137
2.09E+04
8.97E+03
8.97E+01
Cs-138
5.61E+06
2.41E+06
2.41E+04
Cs-139
5.32E+06
2.29E+06
2.29E+04
Cs-140
4.82E+06
2.07E+06
2.07E+04
Sr-89
2.36E+06
1.01E+06
1.01E+04
Sr-90
2.02E+04
8.68E+03
8.68E+01
Sr-91
4.86E+06
2.09E+06
2.09E+04
Sr-92
4.97E+06
2.14E+06
2.14E+04
Sr-93
5.29E+06
2.27E+06
2.27E+04
Sr-94
4.90E+06
2.11E+06
2.11E+04
1.91E+05
4.54E+05
1.10E+03
9.20E+05
1.30E+06
1.65E+06
1.64E+06
1.23E+06
5.41E+05
1.06E+04
7.03E+04
2.41E+06
4.06E+05
1.01E+06
2.14E+06
2.24E+06
1.83E+06
1.29E+06
1.91E+05
4.54E+05
1.10E+03
9.20E+05
1.30E+06
1.65E+06
1.64E+06
1.23E+06
5.41E+05
1.06E+04
7.03E+04
2.41E+06
4.06E+05
1.01E+06
2.14E+06
2.24E+06
1.83E+06
1.29E+06
7.07E+15
1.68E+16
4.07E+13
3.40E+16
4.79E+16
6.12E+16
6.07E+16
4.56E+16
2.00E+16
3.93E+14
2.60E+15
8.92E+16
1.50E+16
3.75E+16
7.93E+16
8.27E+16
6.77E+16
4.77E+16
1.39E-05
5.38E-14
2.52E-04
8.97E-04
2.41E-01
2.29E-01
2.07E-01
1.01E-01
8.68E-04
2.09E-01
2.14E-01
2.27E-01
2.11E-01
1.39E-09
5.38E-18
2.52E-08
8.97E-08
2.41E-05
2.29E-05
2.07E-05
1.01E-05
8.68E-08
2.09E-05
2.14E-05
2.27E-05
2.11E-05
5.15E+01
1.99E-07
9.34E+02
3.32E+03
8.92E+05
8.46E+05
7.67E+05
3.75E+05
3.21E+03
7.74E+05
7.91E+05
8.41E+05
7.79E+05
Downwind
Submersion Dose rate (Sv/h)
Distance
Isotope
I-131 & I- Cs-134
(m)
Krypton Xenon
135
&Cs-137
100
0.00E+00 0.00E+00 0.00E+00 0.00E+00
300
4.02E-16 3.50E-16 3.89E-21 8.19E-26
500
2.86E-08 2.49E-08 2.77E-13 5.83E-18
1000
1.51E-04 1.31E-04 1.46E-09 3.07E-14
1600
8.00E-04 6.96E-04 7.75E-09 1.63E-13
2.4 Estimation of submersion dose rate due to ground release:
Assumption: Leak rate from the containment is assumed 0.2% per hour, wind
speed at the ground 2m/s, up to 200m building wake effect is considered and the
surface area of the building is taken 1400m2, after 200m single plume release is
considered at H=0 with stability class F.
Table 8: Submersion dose rate at different downwind distances for ground release
Downwind
distance
(m)
100m
200m
300m
500m
1000m
1600m
Xe
8.36E-03
7.57E-03
6.68E-03
5.06E-03
3.77E-03
1.77E-03
7.27E-03
6.59E-03
5.81E-03
4.40E-03
3.28E-03
1.54E-03
20
Isotope
I-131 &I135
8.0905E-07
7.3273E-07
2.7471E-06
1.1604E-06
3.647E-07
1.711E-07
Downwind
distance
(m)
100
300
1000
Krypton
2.00E-03
2.41E-03
2.19E-03
Cesium
2.78E-13
3.34E-13
3.01E-13
Table 10: Inhalation dose rate at different downwind distances for stack release
Downwind
distance (m)
100
300
500
1000
1600
Dose rate
(Sv/h)
0.00E+00
9.53E-19
6.78E-11
3.58E-07
1.90E-06
21
2.6.2 From ground release: Leak rate from the containment is assumed 0.2% per
hour, wind speed at the ground 2m/s, up to 500 m building wake effect is
considered and the surface area of the building is taken 1400m2, after 500m single
plume release is considered at H=0 with stability class F.
Table 11: Inhalation dose rate at different downwind distances for ground release
Downwind
distances (m)
100m
200m
300m
500m
1000m
1600m
1.98E-04
1.80E-04
1.58E-04
1.20E-04
8.94E-05
4.19E-05
Table 12: Submersion, plume and inhalation dose rate at different downwind distances
Downwin
d distance
(m)
100
200
300
500
1000
1600
Stack
Release
0.00E+00
7.52E-16
5.35E-08
2.82E-04
1.50E-03
Plume
Dose rate
(Sv/h)
3.68E-03
4.41E-03
3.99E-03
-
22
Stack Release
0.00E+00
9.53E-19
6.78E-11
3.58E-07
1.9E-06
2.7.2 Total dose rate due to submersion, inhalation and plume is estimated for
different downwind distances.
Table 13: Total dose depending on the duration of release at different downwind distances
Downwind
distance
(m)
100
300
1000
30 m
9.75E-03
8.53E-03
5.71E-03
1h
1.95E-02
1.71E-02
1.14E-02
Table 14: Submersion dose rate from stack release in BDBA condition
Downwind
Distance
(m)
Krypton
100
300
500
1000
1600
0.00E+00
4.02E-16
2.86E-08
1.51E-04
8.00E-04
23
Downwind
distance (m)
100
300
1000
Krypton
2.00E-03
2.41E-03
2.19E-03
Cesium
2.78E-13
3.34E-13
3.01E-13
Table 16: Inhalation dose rate from stack release in BDBA condition
Downwind
distance (m)
100
300
500
1000
1600
Dose rate
(Sv/h)
0.00E+00
9.53E-18
6.78E-10
3.58E-06
1.90E-05
24
2.9 Conclusion
The study assumes an hypothetical accident condition in a research reactor
resulting in release of FPNGs, particulate matters and iodine, contributing dose to
the members of the public. Various assumptions in terms of releases are made to
arrive at the dose values and evaluation of dose is made for various modes of
exposure scenarios. From the results, it can be seen that the submersion dose due to
stack release is negligible and that due to ground release is 15.6 mSv at 100 m
downwind distance (see table- 12) and then gradually decreases with increase in
downwind distance. The estimated maximum plume dose is evaluated to be 4.41
mSv at downwind distance 300 m (see table -12). Due to inhalation of iodine, the
evaluated dose is found to be very less. For the BDBA scenario the evaluated dose
only due to iodine is increased by 10% but its contribution to the total dose is
negligible.
It is to be noted that the estimated dose for a hypothetical nuclear accident for a
100 MW research reactor at various downwind distances for different scenarios is
much less than the dose limit specified by AERB for accident conditions.
2.10 References
1. Barratt, R. Atmospheric dispersion modeling: An introduction to practical
applications. (London: Earthscan Publishing Ltd.) (2001).
2. International Commission on Radiological Protection.Compendium of Dose
Coefficients based on ICRP Publication 60.ICRP 119.
3. Martin, J. E. Physics for radiation protection. (2006 WILEY-VCH Verlag GmbH
& Co. KGaA, WeinheimISBN: 3-527-40611-5).
25