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Article history:
Received 31 May 2014
Received in revised form 15 September 2014
Accepted 23 September 2014
Available online xxxx
Keywords:
Hydrothermal mineralization
Singularity
Geo-anomaly
Geographically weighted regression
Spatial non-stationarity
a b s t r a c t
This paper demonstrates a modeling procedure of mineral potential mapping based on singularity theory, and
further presents an idea to look into metallogeny of SnCu polymetallic deposits in southeastern Yunnan mineral
district, China by applying a localized regression method. Mineralization is a typical cascade process generally
accompanied by irregular geological, geochemical and geophysical signatures. Singularity index as an efcient
anomaly analytical tool helps to identify anomalies as well as characterize formation processes of these anomalies. In this study, the singularity-based mineral potential mapping method was utilized to characterize hydrothermal mineralization associated with magmatic, tectonic and sedimentary processes in this district. Based on
the results, a mineral prospectivity model was constructed to delineate target areas. In addition to mineral
prospectivity, controlling effects of geo-processes on mineralization are spatially non-stationary. Geographicallyweighted regression analysis was thus employed to investigate these spatially-varied controlling effects and it
has contributed to improve understanding to local metallogeny in the study area. Results of the spatial analysis
presented can be used to guide following stages of mineral exploration in the district.
2014 Elsevier B.V. All rights reserved.
1. Introduction
The southeastern Yunnan mineral district, China is well-known for
its world class SnCu polymetallic deposits and has attracted great
scientic attentions for decades. A prolonged history of mining activities
in this district can be dated back to 2000 years ago (i.e., the Han dynasty
of China). After the foundation of the P.R. of China, systematical exploration and investigations were signicantly undertaken. In the past
decades, knowledge on types, origins and distributions of SnCu
polymetallic deposits had been greatly improved by deep and detailed
researches (Qin and Li, 2008; Zhuang et al., 1996). Exploration of hydrothermal ore deposits especially the skarn type in this district has been
greatly benetted from improved knowledge on ore genesis and mineral prospectivity modeling (Cheng and Mao, 2010; Cheng et al., 2012,
2013; Liao et al., 2014; Wang et al., 2011, 2012, 2013a, 2013b). Hydrothermal mineralization as a cascade geological process includes migration of ore-bearing hydrothermal uids, metasomatic replacement
between uids and wall rocks, precipitation of minerals and consequent
accumulation of certain elements or metals (Cheng, 2007a; He et al.,
2013; Pirajno, 2009). Concerning the mineralization process discussed
Corresponding author at: State Key Lab of Geological Processes and Mineral Resources,
China University of Geosciences, Beijing 100083, China. Tel.: +86 11 86 10 82323583.
E-mail address: zhaojie.ca@gmail.com (J. Zhao).
above, two main regional ore-controlling factors important to hydrothermal mineralization are tectono-magmatism and wall rocks. The former is crucial since magmatism can provide both ore-forming materials
and heat during mineralization, while tectonism creates spaces for
transportation of magma and/or hydrothermal uids and precipitation
of ore materials (Faulkner et al., 2010; Han et al., 2012; Micklethwaite
et al., 2010; Wang et al., 2013a, 2013b; Yuan et al., 1979; Zhai et al.,
1999; Zhao et al., 2011). The latter, wall rock, is another key factor in hydrothermal mineralization, properties of which are important to types
of mineralization (e.g., skarn type ore deposits formed in contact
zones of felsic intrusions and carbonate rocks) (Chen et al., 2007;
Einaudi and Burt, 1982; Mao et al., 2011). Therefore, detailed researches
on these controlling factors and their controlling effects on mineralization are benecial for mineral potential mapping. Studies regarding to
these points are numerous and so as published literatures. However,
the long and continued exploitation of hydrothermal mineral deposits,
especially skarn-type, had led to the mine crisis in this district. With
the increasing pressure of mine production in recent years, it is necessary to utilize advanced prospectivity analytical techniques and current
knowledge of metallogenesis in the district to assist exploration of
deposits around existing occurrences and toward deeper levels.
Mineral exploration aims to nd economic mineral deposits through
a systematic process consisting of regional area selection, reconnaissance exploration and a series of follow-up surveys (Haldar, 2012;
http://dx.doi.org/10.1016/j.oregeorev.2014.09.032
0169-1368/ 2014 Elsevier B.V. All rights reserved.
Please cite this article as: Wang, W., et al., GIS-based mineral potential modeling by advanced spatial analytical methods in the southeastern
Yunnan mineral district, China, Ore Geol. Rev. (2014), http://dx.doi.org/10.1016/j.oregeorev.2014.09.032
sub-districts Gejiu, BainiuchangWenshang, and DulongMalipofrom the west to the east. Although the study area experienced
a long term geological evolution and its geological framework
is complicated, a general SnCu polymetallic deposit model was
summarized according to systematic studies on diagenesis and
metallogenesis, which greatly supports the mineral prospectivity
modeling (Yang, 1990).
2.1. Geological criteria for modeling
2.1.1. Mineralization process
In former studies (e.g., Guan, 1991; Yang, 1990), a magmatichydrothermal model once was commonly accepted to describe mineralization
of SnCu polymetallic deposits in this district: the Yanshanian granites
with ore-forming materials intruded into carbonate strata, and the
SnCu polymetallic deposits were formed near/in contract zones by
precipitation and crystallization of those ore-forming materials. In recent years, more detailed studies have been conducted, and a conclusion
that the SnCu polymetallic mineralization was related to a complex
metallogenic system dominated by interactions of multi-factor for
multi-stage was suggested (Chen et al., 1998; Li et al., 2005, 2006; Qin
an Li, 2008; Zhang et al., 2006). The SnCu polymetallic mineralization
was brought about by various processes including rift expansion, volcanic sedimentation, marine hydrothermal exhalation, and transformation by granitic intrusions (Fig. 1b). From the Hercynian to the late
Indo-China epochs, inuenced by deep-rooted syngenetic faulting in
the MileShizong and GejiuLuopingQinglong, the study area was in
a rift environment. The volcanic rocks comprise a bimodal suite and
the earliest stratiform Sn, Cu, Pb, and Zn syngenetic sedimentary ores
were formed during this period (Li, 1998; Qin and Li, 2008; Zhou
et al., 1997). In the middle Indo-China epoch, hydrothermal uids carrying ore-forming materials extracted from underlying basement were
developed (Liu et al., 2007a, 2007b; Qin and Li, 2008). Migrated through
fractures, marine volcanic exhalation occurred at the seaoor, which led
to the formation of stratiform and/or lenticular SnCu polymetallic ore
bodies. Tectonic activities during the middle to late Yanshanian epoch
caused large-scale emplacement of granitic magmas in this district,
which are believed to provide parts of ore-forming materials other
than carbonate strata (Li, 1998). In addition, the granitic emplacement
had contributed to the transformation (e.g., alteration, enrichment,
metamorphosis) of existing ore bodies, which caused the formation of
skarn-type sulde ore bodies in irregular and lenticular shapes within
the contact zones between the intrusions and carbonate rocks. Meanwhile, vein and stockwork ore bodies lled up spaces of fractures in
overlying strata as hydrothermal uids cooled down in those fractures
(Qin and Li, 2008).
2.1.2. Mineralization types and controlling factors
Minerals of SnCu polymetallic deposits in the study area are
generally formed following a sequence of early skarn, late skarn,
quartztourmaline (greisens), sulde, and carbonate stages (Yao and
Wu,1988), among which the sulde stage is believed as the main period
of ore-forming element enrichment. The stratiform cassiteritesulde
ore bodies with great economic value are broadly distributed in carbonate rocks. Genesis analysis on these ore bodies suggested the formation
of which are highly associated with the late Yanshanian granitic intrusions (Cheng et al., 2013; Liu et al., 2007a; Luo, 1995; Wang et al.,
2013a; Xiong and Shi, 1994; Zhang et al., 2006; Zhou et al., 1997).
Magmatic activities during the middlelate Yanshanian epoch are
signicant to Sn polymetallic mineralization in the study area. Emplacement of granitic magma dominated the activities and caused the formation of the Gejiu, Bozhushan and Laojunshan intrusions from the west to
the east in the study area (Guan, 1991). The SnCu polymetallic mineralization is annularly occurred around intrusions, intensity of which is
decreased by the distance to intrusions increasing (Guan, 1991; Yao
and Wu, 1988; Yang, 1989; Dai, 1990). Granitic apophyses are often
Please cite this article as: Wang, W., et al., GIS-based mineral potential modeling by advanced spatial analytical methods in the southeastern
Yunnan mineral district, China, Ore Geol. Rev. (2014), http://dx.doi.org/10.1016/j.oregeorev.2014.09.032
a)
b)
c)
Fig. 1. (a) A simplied geological map indicating major geological features of the study area (after Wang, 2004; Wang et al., 2012). F1 = Ailaoshan deep fault. F2 = Red River fault. F3 =
PingJianShi fault. F4 = Xiaojiang fault. F5 = ShizongMile fault. F6 = Nanpanjiang fault. F7 = MengziYanshan fault. F8 = WenshanMalipo fault. F9 = Lvzhijiang fault. (b) A geological map of the southeastern Yunnan mineral district, China. (c) 1 = the Gejiu Formation in the mid-Triassic series. 2 = diabase. 3 = altered granite. 4 = vein ore-bodies. 5 = the Late
Yanshanian granite. 6 = granite. 7 = placer tin deposit. 8 = skarn ore-body. 9 = carbonate rock. 10 = porphyritic granite. 11 = bedded ore-body. 12 = reticular ore-body (after Cheng
et al., 2008).
developed beneath stratiform ore bodies with economic value, and the
concaves between apophyses are favorable positions for mineralization
(Chen et al., 2009; Liu et al., 2007b; Zhou et al., 1997; Zhuang et al.,
1996). Granites in the study area are remelted, Sn contents of which
are much higher than the world average for granites (Li et al., 2005,
2006; Qin et al., 2006a; Zhang et al., 2006; Zhou et al., 1997). Prominent
negative Eu anomalies indicate that the granitic magma was probably
originated from the Crust (Luo, 1995; Mao et al., 2008) and experienced
various degrees of differentiation (Guan, 1993). With increased differentiation of the magma, intensity of Sn mineralization was enhanced
(Qin and Li, 2008; Qin et al., 2004). In other words, the granites in the
study area are highly acidic, strong in activity and prone to react with
wall rocks (Shi, 1984).
Please cite this article as: Wang, W., et al., GIS-based mineral potential modeling by advanced spatial analytical methods in the southeastern
Yunnan mineral district, China, Ore Geol. Rev. (2014), http://dx.doi.org/10.1016/j.oregeorev.2014.09.032
x1
h Ai cA
hC Ai cA
Please cite this article as: Wang, W., et al., GIS-based mineral potential modeling by advanced spatial analytical methods in the southeastern
Yunnan mineral district, China, Ore Geol. Rev. (2014), http://dx.doi.org/10.1016/j.oregeorev.2014.09.032
d A 2
:
dA C A
It implies that the singularity index estimated by the windowbased method is related to the rst derivative transformation of
geophysical elds (A), and the estimation is independent to scales of
A unless the scale independency in Eqs. (1) and (2) does not exist
(Cheng, 2007b, 2008; Wang et al., 2013a).
3.2. Principal component analysis (PCA)
Principal component analysis (PCA) has been broadly used to
integrate geochemical anomalies to delineate spatial distributions of
geological features and mineralization (Carranza and Hale, 2002;
Carranza, 2010; Cheng et al., 2011; Ciampalini et al., 2013; Shahriari
et al., 2013; Wang et al., 2011, 2012, 2013b, 2014a, 2014b; Zhao et al.,
2012, 2013, 2014). It is an efcient statistical technique to reduce
dimensionality of geo-exploratory datasets. Multi-source geo-variables
indicative of the presence of mineralization or its associated geological
features are interrelated in the contexts of both statistical and geological
theories. Based on a coefcient matrix, an orthogonal transformation
constitutes the main algorithm of PCA, by which a series of interrelated
geo-variables are transformed to several uncorrelated geo-variables
termed as principal components (PCs). Each PC is a weighted sum of
all input geo-variables, and the weights (i.e., loadings) of geo-variables
can be interpreted to achieve useful geo-information by geologists.
3.3. Geographically weighted regression (GWR)
Hydrothermal mineralization is a cascade process associated with
various complex geo-processes (i.e., controlling factors) (Cheng,
2008). Interactions among these factors control occurrence of mineralization, variations of which produce different types of ore deposits within certain circumstances. Knowledge regarding this geological issue
exerts inuences on choosing appropriate geological criteria for mineral
potential modeling. From a geo-statistical point of view, the interactions
can be explained by interrelations among geo-information layers descriptive to controlling factors. Regression analysis, which is efcient
in enhancing knowledge regarding dependent (i.e., mineralization)
and independent variables (i.e., controlling factors), can be implemented
to this geological issue (Carranza and Hale, 2001a; Carranza et al., 2008;
Zagayevsky and Deutsch, 2014; Zhao et al., 2013, 2014).
The ordinary least square (OLS) is one of the most popular and
frequently used regression analysis methods, by which interrelations
among controlling factors and mineralization can be expressed as:
Y i a0
ak X ik i
scales across space. Therefore, constant interrelations (ak) among mineralization and its controlling factors generated by OLS are global estimations rather than local ones, which cannot describe detailed and/or
localized situations (Fotheringham et al., 2002; Zhao et al., 2013, 2014).
Focusing on remedying shortages of global regression analysis, geographically weighted regression (GWR), which was proposed to estimate spatially-varied interrelations among variables (Brunsdon et al.,
1996; Fotheringham et al., 1996, 1998), can be introduced to explore
spatially non-stationary controlling effects of geological factors on
mineralization across the space (ui, vi). Thus,
Y i a0 ui ; vi
ak ui ; vi X ik i
0
wi2
0
:
0
0
0
wi3
:
0
0
0
0 :
:
wi j
By using a weighting factor, the jth location is weighted geographically according to its distance to the calibration point i; location j close
to i is dened a higher weight than the ones far from i (Brunsdon
et al., 1996, 2002; Fotheringham et al., 1998, 2001). Meanwhile, a
weight assigned to the jth observation is dependent on a predened
bandwidth . The location j is given a weight exp(dij2/2) if the distance between j and the calibration point i is less than the bandwidth
; otherwise the weigh is 0. In general, a smaller bandwidth produces
more localized investigation on interrelations among mineralization
and its controlling factors, and vice versa. If the bandwidth is approaching innity, weights will become to 1 and estimated interrelations or controlling effects ak(ui, vi) by GWR are same as OLS. More
detailed introduction and geological applications of GWR can be found
in Brunsdon et al. (1996), Fotheringham et al. (2002), and Zhao et al.
(2013, 2014).
4. Mineral exploration modeling
Based on former studies (Zhuang et al., 1996), geo-information regarding the Yanshanian granitic intrusions, intensive faults and carbonate strata are necessary to be extracted and integrated for mineral
potential mapping for SnCu mineralization in the southeastern
Yunnan mineral district, China. Furthermore, in order to investigate
spatially-varied interrelations among mineralization and its controlling
geo-processes, geochemical distributions of ore-forming element
assemblages as end products of hydrothermal mineralization were
characterized by geo-information of the three controlling factors.
4.1. Modeling component recognition
4.1.1. The Yanshanian granitic intrusions
Considering genetic relationships between the Yanshanian granitic
intrusions and SnCu polymetallic hydrothermal deposits in this area,
Please cite this article as: Wang, W., et al., GIS-based mineral potential modeling by advanced spatial analytical methods in the southeastern
Yunnan mineral district, China, Ore Geol. Rev. (2014), http://dx.doi.org/10.1016/j.oregeorev.2014.09.032
a)
b)
Fig. 2. Spatial distributions of singularity indices of geophysical elds (after Wang et al., 2013a). (a) Singularity index of Bouguer; (b) Singularity index of aeromagnetic anomalies.
Please cite this article as: Wang, W., et al., GIS-based mineral potential modeling by advanced spatial analytical methods in the southeastern
Yunnan mineral district, China, Ore Geol. Rev. (2014), http://dx.doi.org/10.1016/j.oregeorev.2014.09.032
a)
0.5
Aeromagnetic data
Bouguer anomalies
b)
Fig. 3. Geo-information extracted from geophysical anomalies. (a) PC1 loadings of singularity indices of gravity and magnetic data supporting that the PC1 depict physical signatures of the
granitic intrusions. (b) Spatial distributions of PC1 scores of singularity indices of Bouguer gravity and aeromagnetic anomalies.
areas with b 2; meanwhile these areas are coincident with well developed fault systems and intersections of faults trending along different
orientations. Details of applications of singularity theory to fault analysis
can be found in our former studies (Wang et al., 2012, 2013b; Zhao et al.,
2013).
4.1.3. Carbonate strata
Stages of hydrothermal mineralization include magmatic emplacement, migration of ore uids through fault systems, hydrothermal
Fig. 4. Spatial distributions of singularity indices of fault density (after Wang et al., 2012). Areas with singularity indices less than 2 correspond to well-developed fault systems.
Please cite this article as: Wang, W., et al., GIS-based mineral potential modeling by advanced spatial analytical methods in the southeastern
Yunnan mineral district, China, Ore Geol. Rev. (2014), http://dx.doi.org/10.1016/j.oregeorev.2014.09.032
a)
b)
Fig. 5. Geochemical signatures of ore-bearing strata characterized by joint application of singularity theory and PCA. (a) PC1 loadings of singularity indices of selected elements and oxides
enriched in carbonate strata. (b) PC1 scores of singularity indices of selected elements and oxides indicating spatial variations of geochemical signatures of ore-bearing strata.
Please cite this article as: Wang, W., et al., GIS-based mineral potential modeling by advanced spatial analytical methods in the southeastern
Yunnan mineral district, China, Ore Geol. Rev. (2014), http://dx.doi.org/10.1016/j.oregeorev.2014.09.032
a)
0.80
0.40
0.00
-0.40
-0.80
Granitic intrusions
Carbonate strata
Fault intensity
b)
Fig. 6. Application of PCA to integrate geo-information identied by singularity theory. (a) Loadings of controlling factors in PC1. (b) PC1 scores, sowing low values indicative of mineral
potentials.
and the hydrothermal mineralization occurred at mineralizationfavored positions within the contract zones between intrusions and
carbonate strata.
4.3. Spatially non-stationary interrelations among mineralization and
controlling factors
Ore-forming elements consisting of Sn, Cu, Pb, As, W, and Zn as end
products of hydrothermal mineralization in southeastern Yunnan mineral district, China are often discontinuously and heterogeneously distributed. To represent hydrothermal mineralization process, spatiallyvaried geochemical behaviors of these elements (i.e., depletion and accumulation) were characterized by singularity theory and further integrated by PCA (Fig. 7). Many discovered that SnCu polymetallic
deposits are located in areas with enrichment of ore-forming element
assemblages (i.e., low PC1 scores) (Fig. 7b). Based on the derived geoinformation regarding the Yanshanian granitic intrusions (Fig. 3b),
fault intensity (Fig. 4) and ore-bearing carbonate strata (Fig. 5b), a
GWR model was constructed to investigate spatially-varied interrelations among hydrothermal mineralization and its controlling factors.
Since high values in Fig. 3 and low values in Figs. 4, 5 and 7 are indicative
of the presence of mineralization, the latter three sets of values were
reclassied so that all high values are coincident with their causative
geological features and in order to facilitate interpretation of the results
of regression analysis. Using geo-anomalies of ore-forming element assemblage as a dependent geo-variable and geo-anomalies of the three
Please cite this article as: Wang, W., et al., GIS-based mineral potential modeling by advanced spatial analytical methods in the southeastern
Yunnan mineral district, China, Ore Geol. Rev. (2014), http://dx.doi.org/10.1016/j.oregeorev.2014.09.032
10
a)
b)
Fig. 7. Spatial distributions of hydrothermal mineralization in the southeastern Yunnan mineral district, China. (a) Loadings of the main ore-forming elements in PC1. (b) PC1 scores
indicative of geochemical behaviors of ore-forming element assemblage. Eight zones with accumulation of ore-forming element assemblage and high density of discovered deposits
are circled for further discussion in the text.
that mineralization is more prone to occur within the outer zones of intrusions in contact with carbonate rocks. Regression residuals depicted
along section YY* represent another signicant variable releasing information for interpretation. Residuals with high values in most zones
(Fig. 8e) imply underestimation of the GWR model as regards mineralization (i.e., dependent variable). In other words, content of ore-forming
element assemblage in high residual areas is much higher than the expectation. Two possible reasons are discussed here. The rst one is
that the residuals are due to intense accumulation of ore-forming element assemblage forced by anomalous geo-processes. It can be proved
by occurrences of known hydrothermal deposits within these areas.
Secondly, there are likely additional local controlling factors which
have not been considered in the GWR model but efciently impact
hydrothermal mineralization or accumulation of relative elements.
Information from either regression coefcients or residuals aids hydrothermal mineral exploration in the study area. Focusing on local
scale, coefcients provide qualitative and quantitative descriptions of
the spatially-varied interrelations among hydrothermal mineralization
and its controlling factors. It benets understanding the metallogeny
of SnCu polymetallic deposits in local areas. Based on these coefcients, the metallogeny can also be rectied in return. Residuals, especially the ones coincident with known mineral occurrences remind
insufciency of the employed model, implying that more localized
metallogeny and detailed exploration should be suggested in these
areas. Therefore, proper interpretation of both regression coefcients
and residuals is necessary and important for mineral exploration in
the study area.
Please cite this article as: Wang, W., et al., GIS-based mineral potential modeling by advanced spatial analytical methods in the southeastern
Yunnan mineral district, China, Ore Geol. Rev. (2014), http://dx.doi.org/10.1016/j.oregeorev.2014.09.032
11
a)
b)
c)
Fig. 8. Spatially non-stationary interrelations between hydrothermal mineralization and its controlling factors investigated by GWR. (a) R2 used to evaluate the tness of the regression
model. (b) Regression coefcients of fault intensity descriptive of controlling effects of fault activities to mineralization. (c) Regression coefcients of ore-bearing strata descriptive of controlling effects of wall rocks on mineralization. (d) Regression coefcients of granitic intrusions descriptive to controlling effects of intrusions on mineralization. (e) Residuals of the GWR model.
Please cite this article as: Wang, W., et al., GIS-based mineral potential modeling by advanced spatial analytical methods in the southeastern
Yunnan mineral district, China, Ore Geol. Rev. (2014), http://dx.doi.org/10.1016/j.oregeorev.2014.09.032
12
d)
e)
Fig. 8 (continued).
Acknowledgment
The authors sincerely thank two anonymous reviewers for their
critical reviews and constructive comments which have improved the
manuscript. This research has been jointly supported by China Geological Survey on New methods for mineral resource potential assessment
(1212010733811) and on Quantitative models for prediction of strategic mineral resources in China (201211022) and Canadian Grants
supported by a NSERC Discovery Research Grant (ERC-OGP0183993).
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Please cite this article as: Wang, W., et al., GIS-based mineral potential modeling by advanced spatial analytical methods in the southeastern
Yunnan mineral district, China, Ore Geol. Rev. (2014), http://dx.doi.org/10.1016/j.oregeorev.2014.09.032