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=
=
0
3
= decay constant = probability of a
nucleus decaying per second
Half-life = time for half the nuclei to
decay
Lifetime (average)
2 ln
2
1
= t
1
=
N
t
4
Units: 1 Becquerel (Bq) = 1
decay/second
1 Curie (Ci) = 3.7 x 10
10
decays/sec (1g of radium)
3 types of radiation emitted
spontaneously
=
4
He nucleus (2 p and 2 n)
= e
or e
+
= high-energy photons (keV,
MeV)
5
Effect of a magnetic field Effect of a magnetic field
B into page
gamma
alpha (+)
beta
X
X
6
Decay rate (Activity)
Half-life e.g.
( ) t N e N
dt
dN
R
t
= = =
0
hr t N
o
1 & 20
2
1
= =
etc
5 2
10 1
20 0
N t (hr)
7
decay decay
8
decay decay
-particle is a
4
He nucleus (2p & 2n)
Z by 2
N by 2
A by 4
+
2
4
2 N
A
Z N
A
Z
Y X
parent daughter
+ Th U
234
90
238
92
yrs t
9
10 47 . 4
2
1
=
9
Disintegration energy Disintegration energy
( )
2
c m M M Q
D P
=
MeV
c m Q
u m M M
u m
u M
u M
Th U
Th
U
275 . 4
502 . 931 004589 . 0
004589 . 0
002602 . 4
043593 . 234
050784 . 238
2
=
= =
=
=
=
=
10
Disintegration energy Disintegration energy
Most of the energy (Q) is KE of
Decay occurs if Q > 0 (energy
released)
Spontaneous decay does not occur if Q
< 0
Conservation of momentum (daughter +
alpha) and Energy gives
( )
|
\
|
=
A
A
Q KE
4
( ) MeV KE U g e 2 . 4
238
234
275 . 4 . .
238
= |
\
|
=
( ) ) (daughter KE KE Q + =
11
Theory of Theory of - -decay decay
Questions to answer:
(1) How do -particles with
KE ~ 4 MeV escape the nucleus
while incoming -particles with
KE ~ 10 MeV are scattered ?
(2) KE() range is ~ 4 to 9 MeV but
half-life varies over 24 orders of
magnitude !
(nanoseconds to billions of years)
12
Theory of Theory of - -decay decay
1911: Geiger & Nuttall noticed
that large Q short half-life
1928: Gamow, Gurney, Condon
et al. QM tunnelling through a
nuclear potential barrier by
The tunnelling model works well,
even though it supposes the to be
preformed inside the nucleus.
Krane 8.3
13
Theory of Theory of - -decay decay
experiences a Coulombic potential
barrier
Z-2
r
{ }
3
1
3
1
) 4 ( 4 2 . 1 ~ ) (
) (
) 2 ( 88 . 2
) (
4
) 2 ( 2
) (
0
2
+
=
=
A fm R
fm r
Z
MeV V
r
e Z
r V
14
Barrier height Barrier height
{ }
MeV
MeV
fm fm R
9 . 27
3 . 9
90 88 . 2
~
) ( height Barrier
3 . 9 234 4 2 . 1 ~ ) (
3
1
3
1
=
= +
+ Th U
234
90
238
92
27.9 MeV
4.2 MeV
9.3 fm
15
Barrier width Barrier width
fm width
fm r
MeV
r
q q
V
4 . 52 3 . 9 7 . 61
7 . 61
2 . 4
4
0
2 1
= =
=
= =
28 MeV
4.2 MeV
9.3 fm
61.7 fm
16
Theory of Theory of - -decay decay
An early triumph of QM was
the Geiger-Nuttall relation
. log log
2
1
Const K n t = +
constant
Livesey 9.44
) log(
2
1
t
) log(
K
17
Theory of Theory of - -decay decay
1
2
2
0
2
0
3
0 2
2
1
1
) ( sinh
) ( 4
1
) (
) ( 2
) (
2
) (
1
2 2
1 1
+ = =
=
=
+ =
=
+ =
R k
E V E
V
A A
F F
T
Fe x
E V m k
De Ce x
mE k
Be Ae x
x ik
x k x k
x ik x ik
h
h
1 2 3
18
Theory of Theory of - -decay decay
2
1
2
1
) ( 98 . 2
4
8
) ( 97 . 3
2
2
exp ~
0
2
0
2
= =
= =
)
`
+
fm
me
b
MeV
m e
a
ZR b
E
Z
a T
h
h
E = energy in MeV
R = radius of daughter in fm
Z = atomic number of parent
19
Theory of Theory of - -decay decay
39
10 6 ) 88 exp(
3 . 9 90 98 . 2
2 . 4
90
97 . 3 exp ~
3 . 9 ~ & 90 , 2 . 4
= =
)
`
+
= =
T
fm R Z MeV E
D
Thus, the probability of an particle
tunnelling out of the nucleus when it
hits the potential barrier is VERY SMALL.
BUT ----- how many times does the hit
the barrier per second ?
i.e. How many escape attempts ?
+ Th U
234
90
238
92
20
Theory of Theory of - -decay decay
v
R
t
2
= Time to cross the nucleus is
Attempt frequency
(knocking rate) is R
v
t
f
2
1
= =
Alpha particle speed = ?
s m
m
E
v
MeV m MeV E
/ 10 4 . 1 ~
2
) 4 . 3727 ( 2 . 4 ~
7
=
=
1 20
15
7
10 5 . 7 ~
10 3 . 9 2
10 4 . 1
= s f
21
Half Half- -life of life of - -decay decay
) 10 46 . 4 expt (
10 9 . 4 10 54 . 1
2 ln
10 5 . 4 10 5 . 7 10 6
9
9 17
1 18 20 39
2
1
2
1
yr
yr s t
t
s
=
= =
= =
=
+ Th U
234
90
238
92
22
Half Half- -life of life of - -decay decay
) 310 expt (
2
10 4 . 3
10 14 . 1
/ 10 06 . 2
10 3 ~
9 . 17 0 . 9 9 . 26 width Barrier
2 . 26 height Barrier
02 . 9
78 . 8
2
1
1 8
1 21
7
13
ns
ns t
s f T
s f
s m v
T
fm fm
MeV
fm R
MeV E
=
=
= =
=
=
= =
=
=
=
+ Pb Po
208
82
212
84
23
decay decay
24
decay decay
-particles are electrons or positrons
(anti-electrons)
Z changes by +1 or 1
N changes by 1 or +1
A is unchanged
+
+
1 1 N
A
Z N
A
Z
Y X
+ N C
14
7
14
6
+
+
+
1 1 N
A
Z N
A
Z
Y X
(Not the whole story see neutrinos)
25
Mechanisms
decay decay
+ e p n
+
+ e n p
n e p +
+
or Electron Capture
an atomic electron
The e
or e
+
is NOT present in the
nucleus prior to decay it is created
during the decay process.
Uncertainty calculation
26
decay decay
MeV Q
d t
e Po Bi
16 . 1
5
2
1
210
84
210
83
=
=
+ +
L
Eisberg & Resnick 16.10
A range of energies !
27
decay decay
The masses of the parent and
daughter nuclei are both fixed so why is
there a range of KE () ?
Problems with Energy
Conservation and Momentum
Conservation
1930: Pauli there must be
another particle involved !
1934: Fermi neutrino
VERY (!) weakly interacting
0 = q
0 m
28
Neutrino in Neutrino in decay decay
Momentum conservation problem
e
cf
e
29
Neutrino Neutrino
Three fermions: all have spin =
Spin angular momentum is not conserved
in the above reaction
The other particle must have spin =
+
+ e n p
e
e n p + +
+ +
:
e
e p n + +
:
Electron-anti-neutrino
Electron-neutrino
Cannot occur for a FREE proton .. ?
Decay of a free neutron. Lifetime ~ 886 s
30
Neutrino detection Neutrino detection
1956: Reines & Cowan
+
+ + e n p
e
+ + Cd Cd Cd n
109 * 109 108
+ +
+
e e
Detect the reaction by detecting the 3 gamma-rays
31
An application of An application of - -decay decay
Carbon Dating Carbon Dating
The ratio of
14
C to
12
C is ~ 1.3 x 10
12
Living organisms exchange CO
2
with
surroundings so ratio is ~ stable.
Exchange stops at death so ratio because
the
14
C decays.
e
e N C + +
14
7
14
6
yrs t 5730
2
1
=
32
25 g charcoal
14
C activity = 250 decays/min
Decay constant
1 12
10 83 . 3
2 ln
2
1
= = s
t
Number of
12
C nuclei in 25 g
24 23
10 26 . 1
12
25
10 02 . 6 = =
( )
12 12 24 14
10 6 . 1 10 3 . 1 10 26 . 1 = =
C N
o
Initial activity (at death)
min / 370 sec / 13 . 6 decays decays N R
o o
= = =
yrs t e
e N R
t
t
3239 370 250
0
= =
=
33
Decay energy Decay energy
( )
( )
( )
2
2
2
:
2 :
:
c M M Q EC
c m M M Q
c M M Q
D P
e D P
D P
=
=
=
+
= dv V V
i f fi
*
Describe the strength of the interaction
with an operator (potential) V
Define a matrix element
The initial and final states are
coupled by the operator V
36
Fermis Golden Rule Fermis Golden Rule
f fi fi
V
2 2
h
=
The transition probability is given by
The nature of the interaction was
unknown at the time !
The density of states can be calculated
in Phase Space : a 6-dim space
defined by 3 spatial coordinates and 3
momentum coordinates
2
e
f
f
p
dE
dp
dp
dn
dE
dn
= =
37
Fermis Golden Rule Fermis Golden Rule
The beta-decay must include both the
electron and the associated anti-
neutrino
2 2
2
p p
dp dp
n d
e
e
=
2 2
) (
e e
e e
E E p
c
dE
dp
c p E E E E
=
+ = + =
Ignores recoil KE of daughter atom.
Assumes neutrino has zero mass
38
(Fermi (Fermi- -) ) Kurie Kurie plot plot
The transition rate is therefore:
) (
) (
2 2
e
e
e e
E E
p
E E p
Krane 9.4
e
p
e
E
Ga
66
Q
39
- -decay, spin & parity decay, spin & parity
Fermi decay: electron and anti-neutrino
spins are antiparallel
No I = = & 0
Gamow-Teller decay: electron and
anti-neutrino spins are parallel
No I = = & 1 , 0
0 0
Except
This assumes that the electron and the anti-
neutrino do not carry orbital angular
momentum
40
- -decay, spin & parity decay, spin & parity
Calculate the decay rate using the Fermi
or the Gamow-Teller mechanisms.
Mirror-decays are mixed transitions:
e
e p n + +
GT F % 82 % 18 +
C N
13
6
13
7
GT F % 24 % 76 +
Non-Mirror-decays are GT-dominant:
GT % 98
41
- -decay mechanism ? decay mechanism ?
(1) V = SCALAR SCALAR
Spatially-dependent terms which are
scalars i.e. independent of direction
No change in parity
Integrand must have EVEN parity to
give a non-zero integral
= dv V V
i f fi
*
f i
& Both EVEN or both ODD
i.e. same parity
42
- -decay mechanism ? decay mechanism ?
(2) V = SCALAR SCALAR
But the spatially-dependent part is a
POLAR vector e.g.
i.e. ODD parity
have different parities
f i
&
r
r
43
- -decay mechanism ? decay mechanism ?
(3) V = AXIAL AXIAL
Contains an AXIAL vector e.g.
Vector product of two polar vectors i.e.
both have ODD parity
So, product has EVEN parity
have same parity f i
&
p r l
r r
r
=
44
- -decay mechanism ? decay mechanism ?
(4) V = PSEUDO PSEUDO- -SCALAR SCALAR
Scalar product of a POLAR and an
AXIAL vector e.g.
Product has ODD parity
have different parities
f i
&
a
r
b b
r r
=
0 > b a
r
r
a a
r r
=
0 <
b a
r
r
b
r
45
- -decay mechanism ? decay mechanism ?
(5) V = VECTOR VECTOR
Scalar product of 2 POLAR vectors
Product has EVEN parity
have same parities
f i
&
) ( ) ( b a b a
r
r
r
r
=
(6) V = TENSOR TENSOR
46
- -decay mechanism ? decay mechanism ?
FERMI model assumed a pure
VECTOR interaction
GAMOW-TELLER assumed a
TENSOR or AXIAL interaction. Takes
into account the spins.
Now we know that the Nuclear WEAK
interaction is Vector-Axial. Strength is
about 10
6
of the Nuclear Strong force.
Later, well look at The Standard Model.
No I = = & 0
No I = = & 1 , 0
47
decay decay
48
decay decay
Isomer a nucleus in an excited
energy state
No change in Z, N or A
Nucleus can also de-excite by
Internal Conversion (excess energy
given to an ATOMIC electron)
+ Ag Ag
m 110 110
free electron
nucleus
atom
49
decay decay
Multipole Radiation: Electric
and Magnetic
Opposite parities
L = 1 Dipole
L = 2 Quadrupole
L = 3 Octupole
L = 4 Hexadecapole etc
1
) 1 ( ) ( & ) 1 ( ) (
+
= =
L L
ML EL
50
decay decay
Transition between nuclear
states:
A multipole of order
transfers angular
momentum per photon
Electric or Magnetic
depends on parities of nuclear
states
f i
I I
L
h L
f i
I L I
r r r
+ =
( ) 4 , 3 , 2 , 1 , ) , ( . .
2
5
2
3
= = L I I g e
f i
( )
f i f i
I I L I I e i + . .
51
decay decay
If there is NO change in parity
between the nuclear states then the
radiation field must have EVEN
parity
If there is a change in parity between
the nuclear states then the radiation
field must have ODD parity
( )
4 , 3 , 2 , 1
4 , 3 , 2 , 1 , ) , (
2
5
2
3
E M E M
L I I
f i
= =
+ +
EVEN PARITY
52
decay decay
You cannot have an L = 0 multipole
(single photon)
The multipolarity correlates with the
angular dependence of the emitted
radiation polarization